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Occurrence and profiles of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) in soils from a typical e-waste recycling area in Southeast China

文献类型：期刊论文

作者Liao, Chunyang1; Lv, Jungang2; Fu, Jianjie2; Zhao, Zongshan2; Liu, Fang1; Xue, Qinzhao1; Jiang, Guibin2
刊名INTERNATIONAL JOURNAL OF ENVIRONMENTAL HEALTH RESEARCH
出版日期2012
卷号22期号:4页码:317-330
关键词E-waste Soil Pahs Pcbs Ocps Residue
ISSN号0960-3123
产权排序[Liao, Chunyang; Liu, Fang; Xue, Qinzhao] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc, Yantai 264003, Peoples R China; [Lv, Jungang; Fu, Jianjie; Zhao, Zongshan; Jiang, Guibin] Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, Beijing 100085, Peoples R China
通讯作者Liao, CY (reprint author), Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc, Yantai 264003, Peoples R China.,cyliao@yic.ac.cn
文献子类Article
英文摘要Surface soils collected from Taizhou, a typical e-waste recycling area in Southeast China, were analyzed for the residues of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), and organochlorine pesticides (OCPs) by using microwave-assisted extraction and gas chromatography -mass spectrometry (GC-MS). The total concentrations of 16 PAHs in US EPA's priority list (Sigma PAHs), six indicator PCBs (Sigma PCBs), 15 OCPs widely used in China (Sigma OCPs) in soils ranged from 125 to 4737 ng/g (average: 854 ng/g), from not detected to 55.4 ng/g (3.16 ng/g), and from 47.9 to 820 ng/g (276 ng/g), respectively. Individual PAHs were ubiquitously found in soil samples with detected ratio of 96% and their residual levels were comparable with those of serious polluted sites. Principal component analysis in combination with diagnostic ratios suggested that the combustion of coal, wood, and plastic wastes that are closely associated with illegal and unsafe recycling operations of e-wastes was the main source of PAHs in this area. Compared with other polluted sites, the PCBs residues in soils were generally low except for those in the major recycling site. The residual levels of OCPs in this region were also relatively higher and hexachlorocyclohexane (HCH), dichlorodiphenyltrichloroethane (DDT) and its metabolite forms including dichlorodiphenyldichloroethane (DDD) and dichlorodiphenyldichloroethylene (DDE), hexachlorobenzene (HCB), and dicofol were dominant species. The composition analysis indicated that the HCHs residues in soils might originate from the application of lindane (pure gamma-HCH) and parts of DDTs possibly from the wide use of dicofol with high impurity of DDT compounds in this region.; Surface soils collected from Taizhou, a typical e-waste recycling area in Southeast China, were analyzed for the residues of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), and organochlorine pesticides (OCPs) by using microwave-assisted extraction and gas chromatography -mass spectrometry (GC-MS). The total concentrations of 16 PAHs in US EPA's priority list (Sigma PAHs), six indicator PCBs (Sigma PCBs), 15 OCPs widely used in China (Sigma OCPs) in soils ranged from 125 to 4737 ng/g (average: 854 ng/g), from not detected to 55.4 ng/g (3.16 ng/g), and from 47.9 to 820 ng/g (276 ng/g), respectively. Individual PAHs were ubiquitously found in soil samples with detected ratio of 96% and their residual levels were comparable with those of serious polluted sites. Principal component analysis in combination with diagnostic ratios suggested that the combustion of coal, wood, and plastic wastes that are closely associated with illegal and unsafe recycling operations of e-wastes was the main source of PAHs in this area. Compared with other polluted sites, the PCBs residues in soils were generally low except for those in the major recycling site. The residual levels of OCPs in this region were also relatively higher and hexachlorocyclohexane (HCH), dichlorodiphenyltrichloroethane (DDT) and its metabolite forms including dichlorodiphenyldichloroethane (DDD) and dichlorodiphenyldichloroethylene (DDE), hexachlorobenzene (HCB), and dicofol were dominant species. The composition analysis indicated that the HCHs residues in soils might originate from the application of lindane (pure gamma-HCH) and parts of DDTs possibly from the wide use of dicofol with high impurity of DDT compounds in this region.
学科主题Environmental Sciences ; Public, Environmental & Occupational Health
WOS关键词ZHEJIANG PROVINCE ; SOURCE APPORTIONMENT ; HEAVY-METALS ; HCH RESIDUES ; HUMAN HEALTH ; RIVER-BASIN ; EAST CHINA ; SEDIMENTS ; DDT ; CONTAMINATION
资助项目Liao, Chunyang; Lv, Jungang; Fu, Jianjie; Zhao, Zongshan; Liu, Fang; Xue, Qinzhao; Jiang, Guibin
WOS研究方向Environmental Sciences & Ecology ; Public, Environmental & Occupational Health
语种英语
WOS记录号WOS:000306743500003
公开日期2013-03-08
源URL[http://ir.yic.ac.cn/handle/133337/6192]  
专题烟台海岸带研究所_污染过程与控制实验室
烟台海岸带研究所_中科院烟台海岸带研究所知识产出
作者单位1.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc, Yantai 264003, Peoples R China
2.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, Beijing 100085, Peoples R China
推荐引用方式
GB/T 7714		 Liao, Chunyang,Lv, Jungang,Fu, Jianjie,et al. Occurrence and profiles of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) in soils from a typical e-waste recycling area in Southeast China[J]. INTERNATIONAL JOURNAL OF ENVIRONMENTAL HEALTH RESEARCH,2012,22(4):317-330.
APA Liao, Chunyang.,Lv, Jungang.,Fu, Jianjie.,Zhao, Zongshan.,Liu, Fang.,...&Jiang, Guibin.(2012).Occurrence and profiles of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) in soils from a typical e-waste recycling area in Southeast China.INTERNATIONAL JOURNAL OF ENVIRONMENTAL HEALTH RESEARCH,22(4),317-330.
MLA Liao, Chunyang,et al."Occurrence and profiles of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) in soils from a typical e-waste recycling area in Southeast China".INTERNATIONAL JOURNAL OF ENVIRONMENTAL HEALTH RESEARCH 22.4(2012):317-330.

入库方式： OAI收割

来源：烟台海岸带研究所

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