Label-free colorimetric detection of tetracycline using analyte-responsive inverse-opal hydrogels based on molecular imprinting technology
文献类型：期刊论文
| 作者 | Yang, Qian1,2; Peng, Hailong1,3; Li, Jinhua2 ; Li, Yanbin3; Xiong, Hua1; Chen, Lingxin2; Xiong, Hua(Nanchang Univ, State Key Lab Food Sci & Technol, Nanchang 330047, Jiangxi, Peoples R China); Chen, Lingxin(Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China)
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| 刊名 | NEW JOURNAL OF CHEMISTRY
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| 出版日期 | 2017-09-21 |
| 卷号 | 41期号:18页码:10174-10180 |
| ISSN号 | 1144-0546 |
| DOI | 10.1039/c7nj02368e |
| 产权排序 | 第2完成单位 |
| 文献子类 | Article |
| 英文摘要 | Novel analyte-responsive inverse-opal hydrogels (IOHs) based on molecular imprinting technology were fabricated to generate a highly selective and sensitive device for the colorimetric detection of tetracycline (TC). The TC-responsive IOHs were constructed by packing periodic silica-air arrays and then photo-polymerizing TC-containing hydrogels between the closely packed silica microspheres. Next, the original silica microspheres were etched, and the TC template molecules were eluted with the remaining hydrogel-air arrays. The abundant imprinted sites in the thin hydrogel walls specifically rebound TC via hydrogen bonds, leading to a periodic spacing change and a Bragg diffraction peak shift that converted the rebinding events into readable optical signals. The TC-responsive IOHs offered favorable linearity over four orders of magnitude (10(-10)-10(-6) mol L-1) with a Bragg diffraction peak blue shift of approximately 43 nm. Excellent recognition selectivity for TC over its analog was also attained. Furthermore, the TC-responsive IOHs were successfully applied to detect TC in food samples of milk and meat, with high recoveries of 88.9-112.0% and 87.0-108.7%, respectively. Using TC as a model, the imprinted analyte-responsive IOHs show great potential as a rapid and cost-effective method for direct, label-free, and sensitive colorimetric measurements of trace pollutants in complicated samples. |
| URL标识 | 查看原文 |
| WOS关键词 | PHOTONIC HYDROGELS ; SENSOR ; POLYMERS ; ANTIBIOTICS ; CHROMATOGRAPHY ; MEMBRANE ; RESIDUES ; SAMPLES ; ARRAYS ; MODE |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000411767400067 |
| 资助机构 | National Natural Science Foundation of China(21667018, 21477160, 31660482) |
| 源URL | [http://ir.yic.ac.cn/handle/133337/23448]  |
| 专题 | 烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室 |
| 通讯作者 | Xiong, Hua; Chen, Lingxin; Xiong, Hua(Nanchang Univ, State Key Lab Food Sci & Technol, Nanchang 330047, Jiangxi, Peoples R China); Chen, Lingxin(Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China) |
| 作者单位 | 1.Nanchang Univ, State Key Lab Food Sci & Technol, Nanchang 330047, Jiangxi, Peoples R China 2.Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China 3.Univ Arkansas, Dept Biol & Agr Engn, Fayetteville, AR 72701 USA |
| 推荐引用方式 GB/T 7714 | Yang, Qian,Peng, Hailong,Li, Jinhua,et al. Label-free colorimetric detection of tetracycline using analyte-responsive inverse-opal hydrogels based on molecular imprinting technology[J]. NEW JOURNAL OF CHEMISTRY,2017,41(18):10174-10180. |
| APA | Yang, Qian.,Peng, Hailong.,Li, Jinhua.,Li, Yanbin.,Xiong, Hua.,...&Chen, Lingxin.(2017).Label-free colorimetric detection of tetracycline using analyte-responsive inverse-opal hydrogels based on molecular imprinting technology.NEW JOURNAL OF CHEMISTRY,41(18),10174-10180. |
| MLA | Yang, Qian,et al."Label-free colorimetric detection of tetracycline using analyte-responsive inverse-opal hydrogels based on molecular imprinting technology".NEW JOURNAL OF CHEMISTRY 41.18(2017):10174-10180. |
入库方式： OAI收割
来源：烟台海岸带研究所
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