Harmonizing Aerosol Carbon Measurements between Two Conventional Thermal/Optical Analysis Methods
文献类型：期刊论文
| 作者 | Zhi, Guorui1; Chen, Yingjun3; Sun, Junying1; Chen, Laiguo4; Tian, Wenjuan5; Duan, Jingchun6; Zhang, Gan2; Chai, Fahe6; Sheng, Guoying2; Fu, Jiamo |
| 刊名 | ENVIRONMENTAL SCIENCE & TECHNOLOGY
 |
| 出版日期 | 2011-04-01 |
| 卷号 | 45期号:7页码:2902-2908 |
| 关键词 | Secondary Organic Aerosol Thermal-optical Analysis Elemental Carbon Particulate Matter Black Carbon Chemical-composition Source Apportionment Temperature Particles Air |
| ISSN号 | 0013-936X |
| 产权排序 | [Zhi, Guorui; Sun, Junying] Chinese Acad Meteorol Sci, Beijing 100081, Peoples R China; [Zhang, Gan; Sheng, Guoying] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China; [Chen, Yingjun] CAS, Yantai Inst Coastal Zone Res Sustainable Dev, Yantai 264003, Shandong, Peoples R China; [Chen, Laiguo] Minist Environm Protect, S China Inst Environm Sci, Guangzhou 510655, Guangdong, Peoples R China; [Tian, Wenjuan] S China Univ Technol, Coll Environm Sci & Engn, Guangzhou 510640, Guangdong, Peoples R China; [Duan, Jingchun; Chai, Fahe] Chinese Res Inst Environm Sci, Beijing 100012, Peoples R China |
| 通讯作者 | Zhi, GR, Chinese Acad Meteorol Sci, Beijing 100081, Peoples R China.zhigr68@yahoo.com.cn ; yjchen@yic.ac.cn |
| 文献子类 | Article |
| 英文摘要 | Although total carbon (TC) can be consistently quantified by various aerosol carbon measurement methods, the demarcation of TC into organic carbon (OC) and elemental carbon (EC) has long been inconsistent. The NIOSH and IMPROVE protocols are most widely used for thermal/optical analysis (TOA), but current knowledge rests in the description that the NIOSH protocol usually gives lower EC values than does the IMPROVE protocol. This study seeks to explore the possibility of quantitatively linking the difference between the two TOA protocols. Residential coal-burning samples that had been collected and analyzed following the NIOSH protocol in previous studies were directly reanalyzed following the IMPROVE protocol for this study. A comparison of each pair of NIOSH and IMPROVE EC values reveals the dynamic relation between the two protocols, which can be expressed as a regression equation, y = (1-x)/(1 + 4.86x(2)) (R-2 = 0.96), where the independent x is the EC/TC ratio (R-EC/TC) for the IMPROVE protocol, and the dependent y is the difference between IMPROVE and NIOSH R-EC/TC relative to IMPROVE R-EC/TC. This regression equation may be the first effort in formulating the relationship between the two TOA protocols, and it is very helpful in harmonizing inconsistent TOA measurements, for example, source characterization, ambient monitoring, and atmospheric modeling.; Although total carbon (TC) can be consistently quantified by various aerosol carbon measurement methods, the demarcation of TC into organic carbon (OC) and elemental carbon (EC) has long been inconsistent. The NIOSH and IMPROVE protocols are most widely used for thermal/optical analysis (TOA), but current knowledge rests in the description that the NIOSH protocol usually gives lower EC values than does the IMPROVE protocol. This study seeks to explore the possibility of quantitatively linking the difference between the two TOA protocols. Residential coal-burning samples that had been collected and analyzed following the NIOSH protocol in previous studies were directly reanalyzed following the IMPROVE protocol for this study. A comparison of each pair of NIOSH and IMPROVE EC values reveals the dynamic relation between the two protocols, which can be expressed as a regression equation, y = (1-x)/(1 + 4.86x(2)) (R-2 = 0.96), where the independent x is the EC/TC ratio (R-EC/TC) for the IMPROVE protocol, and the dependent y is the difference between IMPROVE and NIOSH R-EC/TC relative to IMPROVE R-EC/TC. This regression equation may be the first effort in formulating the relationship between the two TOA protocols, and it is very helpful in harmonizing inconsistent TOA measurements, for example, source characterization, ambient monitoring, and atmospheric modeling. |
| 学科主题 | Engineering, Environmental ; Environmental Sciences |
| WOS关键词 | SECONDARY ORGANIC AEROSOL ; THERMAL-OPTICAL ANALYSIS ; ELEMENTAL CARBON ; PARTICULATE MATTER ; BLACK CARBON ; CHEMICAL-COMPOSITION ; SOURCE APPORTIONMENT ; TEMPERATURE ; PARTICLES ; AIR |
| WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:000288841500059 |
| 资助机构 | National Natural Science Foundations of China [40605033, 40773047, 40973071]; CAS [KZCX2-YW-Q07-04, KZCX2-YW-QN210, KZCX1-YW-06]; Department of Science and Technology of Shandong Province [2007GG2QT06018] |
| 公开日期 | 2011-07-22 |
| 源URL | [http://ir.yic.ac.cn/handle/133337/4898]  |
| 专题 | 烟台海岸带研究所_污染过程与控制实验室 |
| 作者单位 | 1.Chinese Acad Meteorol Sci, Beijing 100081, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China 3.Chinese Acad Sci, Yantai Inst Coastal Zone Res Sustainable Dev, Yantai 264003, Shandong, Peoples R China 4.Minist Environm Protect, S China Inst Environm Sci, Guangzhou 510655, Guangdong, Peoples R China 5.S China Univ Technol, Coll Environm Sci & Engn, Guangzhou 510640, Guangdong, Peoples R China 6.Chinese Res Inst Environm Sci, Beijing 100012, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhi, Guorui,Chen, Yingjun,Sun, Junying,et al. Harmonizing Aerosol Carbon Measurements between Two Conventional Thermal/Optical Analysis Methods[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2011,45(7):2902-2908. |
| APA | Zhi, Guorui.,Chen, Yingjun.,Sun, Junying.,Chen, Laiguo.,Tian, Wenjuan.,...&Fu, Jiamo.(2011).Harmonizing Aerosol Carbon Measurements between Two Conventional Thermal/Optical Analysis Methods.ENVIRONMENTAL SCIENCE & TECHNOLOGY,45(7),2902-2908. |
| MLA | Zhi, Guorui,et al."Harmonizing Aerosol Carbon Measurements between Two Conventional Thermal/Optical Analysis Methods".ENVIRONMENTAL SCIENCE & TECHNOLOGY 45.7(2011):2902-2908. |
入库方式： OAI收割
来源：烟台海岸带研究所
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