Using stable isotopes to trace sources and formation processes of sulfate aerosols from Beijing, China
文献类型：SCI/SSCI论文
| 作者 | Han X. K.; Guo, Q. J.; Liu, C. Q.; Fu, P. Q.; Strauss, H.; Yang, J. X.; Hu, J.; Wei, L. F.; Ren, H.; Peters, M. |
| 发表日期 | 2016 |
| 关键词 | cloud condensation nuclei gas-phase oxidation wet precipitation ammonium-sulfate sulfur isotopes organic-carbon atmosphere fractionation pm2.5 japan |
| 英文摘要 | Particulate pollution from anthropogenic and natural sources is a severe problem in China. Sulfur and oxygen isotopes of aerosol sulfate (delta S-34(sulfate) and delta O-18(sulfate)) and water-soluble ions in aerosols collected from 2012 to 2014 in Beijing are being utilized to identify their sources and assess seasonal trends. The mean delta S-34 value of aerosol sulfate is similar to that of coal from North China, indicating that coal combustion is a significant contributor to atmospheric sulfate. The delta S-34(sulfate) and delta(18)O(sulfate)values are positively correlated and display an obvious seasonality (high in winter and low in summer). Although an influence of meteorological conditions to this seasonality in isotopic composition cannot be ruled out, the isotopic evidence suggests that the observed seasonality reflects temporal variations in the two main contributions to Beijing aerosol sulfate, notably biogenic sulfur emissions in the summer and the increasing coal consumption in winter. Our results clearly reveal that a reduction in the use of fossil fuels and the application of desulfurization technology will be important for effectively reducing sulfur emissions to the Beijing atmosphere. |
| 出处 | Scientific Reports |
| 卷 | 6 |
| 语种 | 英语 |
| ISSN号 | 2045-2322 |
| DOI标识 | 10.1038/srep29958 |
| 源URL | [http://ir.igsnrr.ac.cn/handle/311030/42722]  |
| 专题 | 地理科学与资源研究所_历年回溯文献 |
| 推荐引用方式 GB/T 7714 | Han X. K.,Guo, Q. J.,Liu, C. Q.,et al. Using stable isotopes to trace sources and formation processes of sulfate aerosols from Beijing, China. 2016. |
入库方式： OAI收割
来源：地理科学与资源研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。