In mountainous areas, surface solar radiation (SSR) exhibits high spatiotemporal variation at different slopes and aspects due to its great topographic relief. To get mountain SSR spatial distribution, remote sensing-based methods have been popularly used, which separate SSR into direct solar radiation, diffuse sky radiation, and adjacent terrain radiation. However, the methods are highly depended on the atmospheric and angular information derived from different data sources. To clearly address the uncertainties associated with the estimation, this letter conducted a preliminary comparison study by using different atmospheric transmittance models and digital elevation model (DEM) data to retrieve SSR in the Mt. Gongga region. The comparison results indicated that the uncertainty of the atmospheric constituent data greatly limited the performance of the physical atmospheric transmittance models. The resolution of DEM data also played an important role in SSR determination because of the determination of surface angular information. High-resolution (30-m) DEM data showed better performance than low one (90 m). In addition, the systematic underestimation of SSR estimation with the empirical model was significantly improved by using the averaging method with nearby pixel values. It indicated that the geometric errors of satellite image and DEM data should be considered in the estimation.