中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Stretch-Driven Increase in Ultrahigh Thermal Conductance of Hydrogenated Borophene and Dimensionality Crossover in Phonon Transmission

文献类型:期刊论文

作者Li, Dengfeng1; He, Jia1; Ding, Guangqian1; Tang, QiQi1; Ying, Yan1; He, Junjie1; Zhong, Chengyong1; Liu, Yi1; Feng, Chunbao1; Sun, Qilong2
刊名ADVANCED FUNCTIONAL MATERIALS
出版日期2018-08-01
卷号28期号:31页码:7
ISSN号1616-301X
关键词Borophene Phonon Dispersion Phonon Transmission Strain Effect Thermal Conductance
DOI10.1002/adfm.201801685
英文摘要

Inspirited by the wide range of applications of graphene and the similarity between boron and carbon, 2D boron sheets have gained extensive research interest. In this work, using first-principles combined with a nonequilibrium Green's function method, thermal conductance of fully hydrogenated borophene, named borophane, is studied. Interestingly and in contrast to widely perceived sense, at 300 K, it is found that the thermal conductance of borophane in the armchair direction is remarkably larger than that of graphene. More interesting, a dimensionality crossover is observed in phonon transmission where low-frequency phonons exhibit 2D characteristic, while high-frequency phonons behave like a 1D system, oriented along armchair direction, which results in the ultrahigh thermal conductance. An anomalous increase of thermal conductance with uniaxial tensile strain is observed, which is well explained by the unique puckered structure and chemical bonding in borophane. The excellent in-plane stiffness and flexibility together with the high thermal conductance suggest that borophane is promising for soft thermal channel. Moreover, this unique dimensionality crossover in phonon transmission offers a perfect platform for studying the effect of phonon population in mode space, which is of primary importance for thermal transport in low-dimensional systems.

资助项目National Natural Science Foundation of China[11604035] ; Science and Engineering Research Council[152-70-00017]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
语种英语
出版者WILEY-V C H VERLAG GMBH
WOS记录号WOS:000440283900015
源URL[http://119.78.100.138/handle/2HOD01W0/6561]  
专题高性能计算应用研究中心
作者单位1.Chongqing Univ Posts & Telecommun, Sch Sci, Chongqing 400065, Peoples R China
2.Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China
3.ASTAR, Inst High Performance Comp, Singapore 138632, Singapore
推荐引用方式
GB/T 7714
Li, Dengfeng,He, Jia,Ding, Guangqian,et al. Stretch-Driven Increase in Ultrahigh Thermal Conductance of Hydrogenated Borophene and Dimensionality Crossover in Phonon Transmission[J]. ADVANCED FUNCTIONAL MATERIALS,2018,28(31):7.
APA Li, Dengfeng.,He, Jia.,Ding, Guangqian.,Tang, QiQi.,Ying, Yan.,...&Zhang, Gang.(2018).Stretch-Driven Increase in Ultrahigh Thermal Conductance of Hydrogenated Borophene and Dimensionality Crossover in Phonon Transmission.ADVANCED FUNCTIONAL MATERIALS,28(31),7.
MLA Li, Dengfeng,et al."Stretch-Driven Increase in Ultrahigh Thermal Conductance of Hydrogenated Borophene and Dimensionality Crossover in Phonon Transmission".ADVANCED FUNCTIONAL MATERIALS 28.31(2018):7.

入库方式: OAI收割

来源:重庆绿色智能技术研究院

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