We have numerically demonstrated chiral metamaterials based on double-layered asymmetric U-shape split ring resonators. Dual-band circular dichroism is found in the whole frequency regime from 50 to 250 THz by studying the transmission properties. Huge optical activity and the induced negative refractive index are obtained at resonance by calculating the optical activity and ellipticity of the transmitted E-fields. Chirality parameter and effective refractive index are retrieved to illustrate the tunable optical properties of the metamaterials. The underlying mechanisms for the observed circular clichroism are analyzed. These metamaterials would offer flexible electromagnetic applications in the infrared regime. (C) 2015 Elsevier B.V. All rights reserved.