中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
PM2.5 mass, chemical composition, and light extinction before and during the 2008 Beijing Olympics

文献类型:期刊论文

作者Li, Xinghua1; He, Kebin2; Li, Chengcai3; Yang, Fumo4; Zhao, Qing2; Ma, Yongliang2; Cheng, Yuan2; Ouyang, Wenjuan4; Chen, Gangcai5
刊名JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
出版日期2013-11-16
卷号118期号:21页码:12158-12167
ISSN号2169-897X
DOI10.1002/2013JD020106
通讯作者Yang, FM (reprint author), Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Key Lab Reservoir Aquat Environm, Chongqing 401122, Peoples R China.
英文摘要Distinct contrast of air quality and visibility before and during the 2008 Beijing Olympic Games provides a rare opportunity to investigate the links between PM2.5 mass, chemical composition, and light extinction in this megacity. Twenty-four hour integrated PM2.5 samples were collected, and light scattering coefficients and the concentrations of black carbon were measured at urban Beijing for this purpose during a measurement campaign from 1 July to 20 September 2008, which was classed into four stages according to the levels of emission control measures. Daily PM2.5 concentrations ranged from 15.9 to 156.7 mu g m(-3) with an average of 66.0 +/- 35.1 mu g m(-3). The average PM2.5 mass during the Olympics decreased by 49% from the second stage (20 July to 7 August), mainly due to the reduction of secondary inorganic aerosols (i.e., sulfate, nitrate, and ammonium (SNA)). The counterintuitive increase of PM2.5 mass (by 27% on average) during the second stage with two most serious haze episodes, although more rigorous emission control measures were in place, compared to the first stage (1-19 July), was mainly explained by the unfavorable meteorology and input of sulfate aerosols. A daily PM2.5 mass threshold of 50 mu g m(-3) was extracted for frequent haze occurrence. The extinction fractions of SNA and organic material were each approximately 30% during the 20% best visibility days but changed to 81.7% and 8.4%, respectively, during the 20% worst visibility days. The results indicated that the role of SNA was magnified in haze formation during the 2008 summer in Beijing.
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资助项目National Natural Science Foundation of China (NSFC)[41075093] ; National Natural Science Foundation of China (NSFC)[41375123] ; National Basic Research Program of China[2010CB951803] ; Ministry of Environmental Protection of China[201209007] ; State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex
WOS研究方向Meteorology & Atmospheric Sciences
语种英语
出版者AMER GEOPHYSICAL UNION
WOS记录号WOS:000330611800018
源URL[http://119.78.100.138/handle/2HOD01W0/628]  
专题大气环境研究中心
水质生物转化研究中心
通讯作者Yang, Fumo
作者单位1.Beihang Univ, Sch Chem & Environm, Beijing, Peoples R China
2.Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China
3.Peking Univ, Sch Phys, Beijing 100871, Peoples R China
4.Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Key Lab Reservoir Aquat Environm, Chongqing 401122, Peoples R China
5.Chongqing Inst Environm Sci, Chongqing, Peoples R China
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Li, Xinghua,He, Kebin,Li, Chengcai,et al. PM2.5 mass, chemical composition, and light extinction before and during the 2008 Beijing Olympics[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2013,118(21):12158-12167.
APA Li, Xinghua.,He, Kebin.,Li, Chengcai.,Yang, Fumo.,Zhao, Qing.,...&Chen, Gangcai.(2013).PM2.5 mass, chemical composition, and light extinction before and during the 2008 Beijing Olympics.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,118(21),12158-12167.
MLA Li, Xinghua,et al."PM2.5 mass, chemical composition, and light extinction before and during the 2008 Beijing Olympics".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 118.21(2013):12158-12167.

入库方式: OAI收割

来源:重庆绿色智能技术研究院

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