Characteristics of Carbonaceous Aerosol in PM2.5 at Wanzhou in the Southwest of China
文献类型：期刊论文
| 作者 | Huang, Yimin1; Liu, Yuan2 ; Zhang, Liuyi1,2; Peng, Chao2; Yang, Fumo1,2
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| 刊名 | ATMOSPHERE
 |
| 出版日期 | 2018-02-01 |
| 卷号 | 9期号:2页码:15 |
| 关键词 | fine particle organic carbon elemental carbon secondary organic carbon |
| ISSN号 | 2073-4433 |
| DOI | 10.3390/atmos9020037 |
| 英文摘要 | Hourly organic carbon (OC) and elemental carbon (EC) concentrations in PM2.5 were measured from June 2013 to May 2014 in Wanzhou, the second largest city in the Chongqing Municipality, in the southwest of China. Results show that the annual average concentrations of OC and EC were 13.16 +/- 7.98 and 3.12 +/- 1.51 gCm(-3), respectively. Clear seasonal variations of OC and EC concentrations were observed, with their concentrations at minima in summer and maxima in winter. The diel concentration profile of OC and EC presented a bimodal pattern, which was attributed to the cooperative effects of local meteorological conditions and source emissions. The daily average OC/EC ratio ranged from 2.05 to 8.17 with an average of 4.15 for the whole study period. Strong correlations between OC and EC were found in winter and spring, indicating their common sources, while their correlations were poorer in summer and autumn, indicating that the influence of biogenic emissions and secondary organic carbon (SOC) were significant during those seasons. The estimated SOC concentrations were 2.19 +/- 1.55, 7.66 +/- 5.89, 5.79 +/- 3.51, and 3.43 +/- 2.26 gCm(-3), accounting for 29.2%, 52.7%, 27.4%, and 30.5% of total organic carbon in summer, autumn, winter, and spring, respectively. The analysis of back trajectories suggested that high PM2.5, OC, and EC concentrations were associated with air masses originating from or passing over several industrial centers and urban areas in western and northwestern China. Air trajectories from the southeast with short pathways were the dominant trajectories arriving at Wanzhou, indicating that local sources had a big influence on PM2.5, OC, and EC concentrations. |
| 资助项目 | National Natural Science Foundation of China[41375123] ; Chongqing Municipal Education Commission[KJ1501001] ; Chongqing Municipal Education Commission[KJ1501006] ; Wanzhou project[201503049] ; Wanzhou project[2016037] |
| WOS研究方向 | Meteorology & Atmospheric Sciences |
| 语种 | 英语 |
| WOS记录号 | WOS:000427507000003 |
| 出版者 | MDPI |
| 源URL | [http://119.78.100.138/handle/2HOD01W0/6268]  |
| 专题 | 大气环境研究中心 |
| 通讯作者 | Yang, Fumo |
| 作者单位 | 1.Chongqing Three Gorges Univ, Key Lab Water Environm Evolut & Pollut Control Th, Wanzhou, Peoples R China 2.Chinese Acad Sci, CAS Key Lab Reservoir Environm, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China |
| 推荐引用方式 GB/T 7714 | Huang, Yimin,Liu, Yuan,Zhang, Liuyi,et al. Characteristics of Carbonaceous Aerosol in PM2.5 at Wanzhou in the Southwest of China[J]. ATMOSPHERE,2018,9(2):15. |
| APA | Huang, Yimin,Liu, Yuan,Zhang, Liuyi,Peng, Chao,&Yang, Fumo.(2018).Characteristics of Carbonaceous Aerosol in PM2.5 at Wanzhou in the Southwest of China.ATMOSPHERE,9(2),15. |
| MLA | Huang, Yimin,et al."Characteristics of Carbonaceous Aerosol in PM2.5 at Wanzhou in the Southwest of China".ATMOSPHERE 9.2(2018):15. |
入库方式： OAI收割
来源：重庆绿色智能技术研究院
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