Effect of H-bond topology on the lifetimes of cagelike water clusters immersed in liquid water and the probability distribution of these lifetimes: Implications for hydrate nucleation mechanisms
文献类型：期刊论文
| 作者 | Guo, GJ; Zhang, YG; Refson, K |
| 刊名 | CHEMICAL PHYSICS LETTERS
 |
| 出版日期 | 2005-09-26 |
| 卷号 | 413期号:4-6页码:415-419 |
| ISSN号 | 0009-2614 |
| DOI | 10.1016/j.cplett.2005.08.015 |
| 文献子类 | Article |
| 英文摘要 | We perform molecular dynamics simulations to study whether the H-bond topology affects the lifetimes of cagelike water clusters immersed in liquid water. Six clusters with H-bond topologies of different energy levels are considered. The lifetimes of each cluster are measured 200 times independently. Statistical analyses show that the H-bond topology has no effect on the lifetimes and the lifetime data obey the lognormal distribution. The implications of these results for the studies on gas hydrate nucleation mechanisms are discussed. (c) 2005 Elsevier B.V. All rights reserved. |
| WOS关键词 | MOLECULAR-DYNAMICS ; HYDROGEN ; SIMULATION ; DISSOCIATION ; FRAMEWORKS ; (H2O)(20) ; MODEL ; FORM |
| WOS研究方向 | Chemistry ; Physics |
| 语种 | 英语 |
| WOS记录号 | WOS:000232094200032 |
| 出版者 | ELSEVIER SCIENCE BV |
| 源URL | [http://ir.iggcas.ac.cn/handle/132A11/65013]  |
| 专题 | 中国科学院地质与地球物理研究所 |
| 通讯作者 | Guo, GJ |
| 作者单位 | 1.Chinese Acad Sci, Inst Geol & Geophys, State Key Lab Lithopher Evolut, Beijing 100029, Peoples R China 2.Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England |
| 推荐引用方式 GB/T 7714 | Guo, GJ,Zhang, YG,Refson, K. Effect of H-bond topology on the lifetimes of cagelike water clusters immersed in liquid water and the probability distribution of these lifetimes: Implications for hydrate nucleation mechanisms[J]. CHEMICAL PHYSICS LETTERS,2005,413(4-6):415-419. |
| APA | Guo, GJ,Zhang, YG,&Refson, K.(2005).Effect of H-bond topology on the lifetimes of cagelike water clusters immersed in liquid water and the probability distribution of these lifetimes: Implications for hydrate nucleation mechanisms.CHEMICAL PHYSICS LETTERS,413(4-6),415-419. |
| MLA | Guo, GJ,et al."Effect of H-bond topology on the lifetimes of cagelike water clusters immersed in liquid water and the probability distribution of these lifetimes: Implications for hydrate nucleation mechanisms".CHEMICAL PHYSICS LETTERS 413.4-6(2005):415-419. |
入库方式： OAI收割
来源：地质与地球物理研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。