New strategies for submicron characterization the carbon binding of reactive minerals in long-term contrasting fertilized soils: implications for soil carbon storage
文献类型：期刊论文
| 作者 | Xiao, Jian1,8; He, Xinhua2,3; Hao, Jialong4; Zhou, Ying5; Zheng, Lirong5,6; Ran, Wei1; Shen, Qirong1; Yu, Guanghui1,7 |
| 刊名 | BIOGEOSCIENCES
 |
| 出版日期 | 2016 |
| 卷号 | 13期号:12页码:3607-3618 |
| DOI | 10.5194/bg-13-3607-2016 |
| 文献子类 | Article |
| 英文摘要 | Mineral binding is a major mechanism for soil carbon (C) stabilization. However, the submicron information about the in situ mechanisms of different fertilization practices affecting organo-mineral complexes and associated C preservation remains unclear. Here, we applied nano-scale secondary ion mass spectrometry (NanoSIMS), X-ray photoelectron spectroscopy (XPS), and X-ray absorption fine structure spectroscopy (XAFS) to examine differentiating effects of inorganic versus organic fertilization on interactions between highly reactive minerals and soil C preservation. To examine such interactions, soils and their extracted colloids were collected during a 24-year long-term fertilization period (1990-2014) (no fertilization, control; chemical nitrogen (N), phosphorus (P), and potassium (K) fertilization, NPK; and NPK plus swine manure fertilization, NPKM). The results for different fertilization conditions showed a ranked soil organic matter concentration with NPKM > aEuro-NPKaEuro-> aEuro-control. Meanwhile, oxalate-extracted Al (Al-o), Fe (Fe-o), short-range ordered Al (Al-xps), Fe (Fe-xps), and dissolved organic carbon (DOC) ranked with NPKM > aEuro-controlaEuro-> aEuro-NPK, but the ratios of DOCaEuro-a center dot aEuro-Al-xps and DOCaEuro-a center dot aEuro-Fe-xps ranked with NPKMaEuro-> aEuro-NPKaEuro-> aEuro-control. Compared with the NPK treatment, the NPKM treatment enhanced the C-binding loadings of Al and Fe minerals in soil colloids at the submicron scale. Furthermore, a greater concentration of highly reactive Al and Fe minerals was presented under NPKM than under NPK. Together, these submicron-scale findings suggest that both the reactive mineral species and their associations with C are differentially affected by 24-year long-term inorganic and organic fertilization. |
| WOS关键词 | DISSOLVED ORGANIC-MATTER ; RAY PHOTOELECTRON-SPECTROSCOPY ; ION MASS-SPECTROMETRY ; PHOSPHORUS SPECIATION ; MANURE APPLICATION ; MICROBIAL CARBON ; ASSOCIATIONS ; COLLOIDS ; SCALE ; MICROSCOPY |
| WOS研究方向 | Environmental Sciences & Ecology ; Geology |
| 语种 | 英语 |
| WOS记录号 | WOS:000379427700006 |
| 资助机构 | National Natural Science Foundation of China(41371248 ; National Natural Science Foundation of China(41371248 ; Natural Science Foundation of Jiangsu Province of China(BK20131321) ; Natural Science Foundation of Jiangsu Province of China(BK20131321) ; Qing Lan Project ; Qing Lan Project ; Innovative Research Team Development Plan of the Ministry of China(IRT1256) ; Innovative Research Team Development Plan of the Ministry of China(IRT1256) ; 111 Project(B12009) ; 111 Project(B12009) ; Priority Academic Program Development (PAPD) of Jiangsu Higher Education Institutions ; Priority Academic Program Development (PAPD) of Jiangsu Higher Education Institutions ; Shanghai Municipal Bureau of Quality and Technical Supervision(2014-02) ; Shanghai Municipal Bureau of Quality and Technical Supervision(2014-02) ; 41371299) ; 41371299) ; National Natural Science Foundation of China(41371248 ; National Natural Science Foundation of China(41371248 ; Natural Science Foundation of Jiangsu Province of China(BK20131321) ; Natural Science Foundation of Jiangsu Province of China(BK20131321) ; Qing Lan Project ; Qing Lan Project ; Innovative Research Team Development Plan of the Ministry of China(IRT1256) ; Innovative Research Team Development Plan of the Ministry of China(IRT1256) ; 111 Project(B12009) ; 111 Project(B12009) ; Priority Academic Program Development (PAPD) of Jiangsu Higher Education Institutions ; Priority Academic Program Development (PAPD) of Jiangsu Higher Education Institutions ; Shanghai Municipal Bureau of Quality and Technical Supervision(2014-02) ; Shanghai Municipal Bureau of Quality and Technical Supervision(2014-02) ; 41371299) ; 41371299) |
| 源URL | [http://ir.iggcas.ac.cn/handle/132A11/13785]  |
| 专题 | 地质与地球物理研究所_科技支撑系统 |
| 作者单位 | 1.Nanjing Agr Univ, Jiangsu Collaborat Innovat Ctr Solid Organ Waste, Jiangsu Prov Key Lab Organ Solid Waste Utilizat, Natl Engn Res Ctr Organ Based Fertilizers, Nanjing 210095, Jiangsu, Peoples R China 2.Southwest Univ, Coll Resources & Environm, Ctr Excellence Soil Biol, Chongqing 400715, Peoples R China 3.Univ Western Australia, Sch Plant Biol, Crawley, WA 6009, Australia 4.Chinese Acad Sci, Inst Geol & Geophys, Key Lab Earth & Planetary Phys, Beijing 100029, Peoples R China 5.Shanghai Inst Measurement & Testing Technol, Shanghai 201203, Peoples R China 6.Chinese Acad Sci, Beijing Synchrotron Radiat Facil, Inst High Energy Phys, Beijing 100049, Peoples R China 7.N Carolina State Univ, Dept Plant Pathol, Box 7616, Raleigh, NC 27695 USA 8.Columbia Univ, Dept Earth & Environm Engn, New York, NY 10027 USA |
| 推荐引用方式 GB/T 7714 | Xiao, Jian,He, Xinhua,Hao, Jialong,et al. New strategies for submicron characterization the carbon binding of reactive minerals in long-term contrasting fertilized soils: implications for soil carbon storage[J]. BIOGEOSCIENCES,2016,13(12):3607-3618. |
| APA | Xiao, Jian.,He, Xinhua.,Hao, Jialong.,Zhou, Ying.,Zheng, Lirong.,...&Yu, Guanghui.(2016).New strategies for submicron characterization the carbon binding of reactive minerals in long-term contrasting fertilized soils: implications for soil carbon storage.BIOGEOSCIENCES,13(12),3607-3618. |
| MLA | Xiao, Jian,et al."New strategies for submicron characterization the carbon binding of reactive minerals in long-term contrasting fertilized soils: implications for soil carbon storage".BIOGEOSCIENCES 13.12(2016):3607-3618. |
入库方式： OAI收割
来源：地质与地球物理研究所
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