中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
首页 机构 成果 学者
  
  1. CAS IR Grid
  2. 地质与地球物理研究所
  3. 中国科学院地质与地球物理研究所
  4. 兰州油气中心
Hydrocarbon generation and potential in continental organic-rich shales at the highly-mature stage, as determined by hydrous pyrolysis under supercritical conditions

文献类型：期刊论文

作者Wu, Yuandong1,2; Zhang, Zhongning1; Sun, Lina3; Li, Yuanju1,4; He, Cong1; Ji, Liming1; Su, Long1; Zhang, Dongwei1,4
刊名INTERNATIONAL JOURNAL OF COAL GEOLOGY
出版日期2018-02-15
卷号187页码:83-93
关键词Hydrous Pyrolysis Continental Shale Hydrocarbon Generation High Maturity Hydrocarbon Potential Semi-closed System
ISSN号0166-5162
DOI10.1016/j.coal.2018.01.006
文献子类Article
英文摘要Hydrous pyrolysis experiments were conducted to assess hydrocarbon generation and potential in three continental organic-rich shales at the highly-mature stage. The results of this study have important implications for deep petroleum exploration in China. The calcareous shale dominated by type-I kerogen reached its peak oil generation at a vitrinite reflectance (VR) of 1.5 %R-o, and entered the major stage of gas generation at a VR ranging from 1.50 to 2.44 %R-o. The high HI, low S-2 and low atomic H/C ratio revealed that the calcareous shale has some potential for hydrocarbon generation at a VR greater than 2.44 %R-o. The mudstone with type-II kerogen reached its peak oil generation at a VR of 2.5 %R-o. The high atomic H/C ratio, but low HI and S-2 indicated that mudstone may retain some hydrocarbon potential. The carbonaceous mudstone dominated by type-III kerogen had still not reached its peak of hydrocarbon generation at a VR of 3.12 %R-o. The low dryness of the gaseous hydrocarbon yields shows that the carbonaceous mudstone was still in the primary gas generation stage. The high values of S-2 and atomic H/C fraction, but low HI, revealed that the carbonaceous mudstone may retain a large hydrocarbon generation potential at higher maturity stages. Our results suggested that the continental type-I and -II kerogen may have potential for shale gas and deep petroleum generation, while the continental type-III kerogen retained good potential for yielding deep natural gas.
WOS关键词ARTIFICIAL MATURATION SERIES ; INDIVIDUAL N-ALKANES ; BOHAI BAY BASIN ; SOURCE ROCKS ; GAS GENERATION ; WATER-PRESSURE ; SICHUAN BASIN ; LIAOHE BASIN ; LABORATORY EXPERIMENTS ; PETROLEUM GENERATION
WOS研究方向Energy & Fuels ; Geology
语种英语
WOS记录号WOS:000427213800008
出版者ELSEVIER SCIENCE BV
资助机构National Science and Technology Major Projects of Ministry of Science and Technology of China(2016ZX05007001-004) ; Key Laboratory Project of Gansu Province(1309RTSA041) ; National Science and Technology Major Projects of Ministry of Science and Technology of China(2016ZX05007001-004) ; Key Laboratory Project of Gansu Province(1309RTSA041) ; National Science and Technology Major Projects of Ministry of Science and Technology of China(2016ZX05007001-004) ; Key Laboratory Project of Gansu Province(1309RTSA041) ; National Science and Technology Major Projects of Ministry of Science and Technology of China(2016ZX05007001-004) ; Key Laboratory Project of Gansu Province(1309RTSA041)
源URL[http://ir.iggcas.ac.cn/handle/132A11/88213]  
专题地质与地球物理研究所_兰州油气中心
通讯作者Zhang, Zhongning
作者单位1.Chinese Acad Sci, Key Lab Petr Resources, Key Lab Petr Resources Res, Inst Geol & Geophys, Lanzhou 730000, Gansu, Peoples R China
2.Powerchina Water Environm Governance, Shenzhen 518102, Peoples R China
3.Yangtze Univ, Hubei Cooperat Innovat Ctr Unconvent Oil & Gas, Wuhan 430100, Hubei, Peoples R China
4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714		 Wu, Yuandong,Zhang, Zhongning,Sun, Lina,et al. Hydrocarbon generation and potential in continental organic-rich shales at the highly-mature stage, as determined by hydrous pyrolysis under supercritical conditions[J]. INTERNATIONAL JOURNAL OF COAL GEOLOGY,2018,187:83-93.
APA Wu, Yuandong.,Zhang, Zhongning.,Sun, Lina.,Li, Yuanju.,He, Cong.,...&Zhang, Dongwei.(2018).Hydrocarbon generation and potential in continental organic-rich shales at the highly-mature stage, as determined by hydrous pyrolysis under supercritical conditions.INTERNATIONAL JOURNAL OF COAL GEOLOGY,187,83-93.
MLA Wu, Yuandong,et al."Hydrocarbon generation and potential in continental organic-rich shales at the highly-mature stage, as determined by hydrous pyrolysis under supercritical conditions".INTERNATIONAL JOURNAL OF COAL GEOLOGY 187(2018):83-93.

入库方式： OAI收割

来源：地质与地球物理研究所

浏览0
下载0
收藏0
其他版本

除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。