Highly efficient visible-light-driven plasmonic photocatalysts based on graphene oxide mediated hybridization of graphite and Ag/AgBr
文献类型：期刊论文
| 作者 | Geng, Guangwei1,2; Guan, Bo2; Chen, Penglei1,2,3; Zhu, Mingshan2; Yang, Changchun1; Liu, Minghua2,3 |
| 刊名 | RSC ADVANCES
 |
| 出版日期 | 2017 |
| 卷号 | 7期号:16页码:9948-9957 |
| 英文摘要 | Graphite (Gr)-based composite materials have been attracting great interest from the scientific and engineering communities. While tremendous progress has been achieved in this field, it still remains a formidable challenge to hybridize pristine Gr with other components under ambient conditions without breaking the p-conjugated system of Gr. Herein, we report that Gr could be facilely hybridized with visible-light-driven plasmonic photocatalyst Ag/AgBr with the assistance of graphene oxide (GO) nanosheets under ambient conditions. We demonstrate that without the use of GO, Gr could not be well hybridized with Ag/AgBr, while a good hybrid Gr/GO/Ag/AgBr could be produced when GO nanosheets are introduced into the system. Our results show that compared to Ag/AgBr, GO/Ag/AgBr and Gr/Ag/AgBr species, thus-fabricated Gr/GO/Ag/AgBr hybrids could display substantially enhanced catalytic activity towards the photobleaching of methyl orange under visible-light irradiation. It is disclosed that the good hybridization between Gr and Ag/AgBr, which is mediated by GO, and the facilitated separation of photogenerated electrons and holes, which is promoted both by GO and Gr, contribute much to the boosted catalytic performances. Considering the excellent hybridization capability of GO, the exceptional electronic characteristics, versatile multifunctionality and low-cost of Gr, our protocol might be applicable not only to the Ag/AgBr-based plasmonic photocatalysts but also to a wide variety of other functional materials, wherein Gr/GO-based advanced materials of desired and reinforced functions or properties might be inaugurated. |
| 语种 | 英语 |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/38070]  |
| 专题 | 化学研究所_胶体、界面与化学热力学实验室 |
| 作者单位 | 1.Zhengzhou Univ, Coll Chem & Mol Engn, 100 Sci Rd, Zhengzhou 450001, Henan, Peoples R China 2.Chinese Acad Sci, Beijing Natl Lab Mol Sci, Inst Chem, 2 Zhongguancun Beiyijie, Beijing 100190, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Geng, Guangwei,Guan, Bo,Chen, Penglei,et al. Highly efficient visible-light-driven plasmonic photocatalysts based on graphene oxide mediated hybridization of graphite and Ag/AgBr[J]. RSC ADVANCES,2017,7(16):9948-9957. |
| APA | Geng, Guangwei,Guan, Bo,Chen, Penglei,Zhu, Mingshan,Yang, Changchun,&Liu, Minghua.(2017).Highly efficient visible-light-driven plasmonic photocatalysts based on graphene oxide mediated hybridization of graphite and Ag/AgBr.RSC ADVANCES,7(16),9948-9957. |
| MLA | Geng, Guangwei,et al."Highly efficient visible-light-driven plasmonic photocatalysts based on graphene oxide mediated hybridization of graphite and Ag/AgBr".RSC ADVANCES 7.16(2017):9948-9957. |
入库方式： OAI收割
来源：化学研究所
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