中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Removal of fluoride from aqueous solution by Mg-Al-Zr triple-metal composite

文献类型:期刊论文

作者Wang, Mei1; Yu, Xiaolin2; Yang, Chongling3; Yang, Xueqin2,4; Lin, Mengya2,4; Guan, Litao1; Ge, Maofa2,5
刊名CHEMICAL ENGINEERING JOURNAL
出版日期2017-08-15
卷号322页码:246-253
关键词Mg-al-zr Triple-metal Composite Fluoride Adsorption Isotherm
英文摘要Mg-Al-Zr triple-metal composite was fabricated by a facile co-precipitation method for fluoride removal. The as-prepared composite was characterized by various technologies. The adsorption experiment was carried out to investigate the fluoride removal performance. The results showed that the uncalcined Mg-Al-Zr composite exhibited the best fluoride removal capacity of 22.9 mg/g from the Langmuir isotherm model. The adsorption kinetics followed the pseudo-second-order model, and the adsorption isotherm could be better described by Langmuir and Freundlich isotherm model. In a wide pH range (3-10), the fluoride adsorption capacity of the composite was relatively high. Adsorption thermodynamics result indicated the adsorption process of fluoride onto Mg-Al-Zr composite was the endothermic reaction. The as-prepared composite exhibited the excellent fluoride removal ability in the real ground water and surface water. Based on the characterization, the fluoride removal mechanism onto the Mg-Al-Zr composite was proposed, including the ion-exchange by hydroxyl group and NO3 and the complexation by hydroxyl group. (C) 2017 Elsevier B.V. All rights reserved.
语种英语
源URL[http://ir.iccas.ac.cn/handle/121111/38387]  
专题化学研究所_分子动态与稳态结构实验室
作者单位1.South China Agr Univ, Coll Mat & Energy, Guangzhou 510642, Guangdong, Peoples R China
2.Chinese Acad Sci, Inst Chem, CAS Res Educ Ctr Excellence Mol Sci, State Key Lab Struct Chem Unstable & Stable Speci, Beijing 100190, Peoples R China
3.Guangdong Ind Tech Coll, Dept Chem Engn, Guangzhou 510300, Guangdong, Peoples R China
4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
5.Chinese Acad Sci, Inst Urban Environm, Ctr Excellence Reg Atmospher Environm, Xiamen 361021, Peoples R China
推荐引用方式
GB/T 7714
Wang, Mei,Yu, Xiaolin,Yang, Chongling,et al. Removal of fluoride from aqueous solution by Mg-Al-Zr triple-metal composite[J]. CHEMICAL ENGINEERING JOURNAL,2017,322:246-253.
APA Wang, Mei.,Yu, Xiaolin.,Yang, Chongling.,Yang, Xueqin.,Lin, Mengya.,...&Ge, Maofa.(2017).Removal of fluoride from aqueous solution by Mg-Al-Zr triple-metal composite.CHEMICAL ENGINEERING JOURNAL,322,246-253.
MLA Wang, Mei,et al."Removal of fluoride from aqueous solution by Mg-Al-Zr triple-metal composite".CHEMICAL ENGINEERING JOURNAL 322(2017):246-253.

入库方式: OAI收割

来源:化学研究所

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