Capillary-Bridge Mediated Assembly of Conjugated Polymer Arrays toward Organic Photodetectors
文献类型:期刊论文
作者 | Gao, Hanfei1,2; Feng, Jiangang1,2; Zhang, Bo1; Xiao, Chengyi4; Wu, Yuchen1; Kan, Xiaonan3; Su, Bin5; Wang, Zhaohui4; Hu, Wenping4; Sun, Yanming6,7 |
刊名 | ADVANCED FUNCTIONAL MATERIALS
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出版日期 | 2017-09-13 |
卷号 | 27期号:34 |
关键词 | 1d Arrays Conjugated Polymers Dewetting Optoelectronics Photodetectors |
英文摘要 | Large-scale patterning of high-quality organic semiconductors is crucial for the fabrication of optoelectronic devices with high efficiency and low cost. Yet, owing to the uncontrollable dewetting dynamics of organic liquid in conventional solution patterning techniques, large defect density of organic architectures is inevitable, which is detrimental to the device performance. To address this challenge, herein a capillary-bridge-mediated assembly technique is developed for regulating the dewetting process, yielding large-scale 1D microstructure ordered arrays. The 1D arrays organic photodetectors exhibit a high optoelectronic performance of light on/off ratio exceeding 100, responsivity of 3.24 A W-1, detectivity of 3.20 x 10(11) Jones and fast response speed, showing a great improvement compared with spin-coated membrane devices. In addition, the significant enhancement of the device photodetection under the electronic field modulation is investigated by applying a back-gate voltage and explained with the photocurrent predominating in the OFF state and the neglected thermocurrent and tunneling current promoting in the ON state of the phototransistor devices. The research offers a new insight for the facile fabrication of large-scale integrated photodetectors and other organic devices based on patterned conjugated polymers. |
语种 | 英语 |
源URL | [http://ir.iccas.ac.cn/handle/121111/39316] ![]() |
专题 | 化学研究所_有机固体实验室 |
作者单位 | 1.Chinese Acad Sci, Tech Inst Phys & Chem, Lab Bioinspired Smart Interface Sci, Beijing 100190, Peoples R China 2.UCAS, Beijing 100049, Peoples R China 3.Qingdao Univ Sci & Technol, Sch Polymer Sci & Engn, Qingdao 266042, Peoples R China 4.Chinese Acad Sci, Inst Chem, Key Lab Organ Solids, BNLMS, Beijing 100190, Peoples R China 5.Monash Univ, Dept Chem Engn, Clayton, Vic 3800, Australia 6.Beihang Univ, Key Lab Bioinspired Smart Interfacial Sci & Techn, Minist Educ,Sch Chem & Environm, Beijing Key Lab Bioinspired Energy Mat & Devices, Beijing 100190, Peoples R China 7.Beihang Univ, Int Res Inst Multidisciplinary Sci, Heeger Beijing Res & Dev Ctr, Beijing 100190, Peoples R China |
推荐引用方式 GB/T 7714 | Gao, Hanfei,Feng, Jiangang,Zhang, Bo,et al. Capillary-Bridge Mediated Assembly of Conjugated Polymer Arrays toward Organic Photodetectors[J]. ADVANCED FUNCTIONAL MATERIALS,2017,27(34). |
APA | Gao, Hanfei.,Feng, Jiangang.,Zhang, Bo.,Xiao, Chengyi.,Wu, Yuchen.,...&Heeger, Alan J..(2017).Capillary-Bridge Mediated Assembly of Conjugated Polymer Arrays toward Organic Photodetectors.ADVANCED FUNCTIONAL MATERIALS,27(34). |
MLA | Gao, Hanfei,et al."Capillary-Bridge Mediated Assembly of Conjugated Polymer Arrays toward Organic Photodetectors".ADVANCED FUNCTIONAL MATERIALS 27.34(2017). |
入库方式: OAI收割
来源:化学研究所
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