Carbon Nanoparticle Hybrid Aerogels: 3D Double-Interconnected Network Porous Microstructure, Thermoelectric, and Solvent-Removal Functions
文献类型：期刊论文
| 作者 | Tan, Dongxing1,2; Zhao, Jian2; Gao, Caiyan1; Wang, Hanfu3; Chen, Guangming1; Shi, Donglu4 |
| 刊名 | ACS APPLIED MATERIALS & INTERFACES
 |
| 出版日期 | 2017-07-05 |
| 卷号 | 9期号:26页码:21820-21828 |
| 关键词 | Reduced Graphene Oxide Carbon Nanotube Aerogel Thermoelectric Solvent Removal |
| 英文摘要 | We report reduced graphene oxide (rGO)/single-walled carbon nanotube (SWCNT) hybrid aerogels with enhanced thermoelectric (TE) performance and removal of organic solvents by designing 3D double interconnected network porous microstructures. A convenient, cost-effective, and scalable preparation procedure is proposed compared with conventional high temperature pyrolysis and supercritical drying techniques. The obtained hybrid aerogels are systematically characterized by apparent density, scanning electron microscopy, X-ray photoemission spectroscopy, Raman spectroscopy, and porosity. An enhanced TE performance of ZT approximate to similar to 8.03 X 10(-3) has been achieved due to the 3D double-interconnected network porous microstructure, the energy filtering effect, and the phonon scattering at the abundant interfaces and joints. In addition, upon a large axial compression deformation, a high degree of retention of the Seebeck coefficient and a simultaneously significant enhancement of the electrical conductivity are observed. Finally, the hybrid aerogels display high capability for the removal of diverse organic solvents and good recyclability. These findings open a new avenue for exploiting aerogels with multifunctions and widening the applications of TE materials by judicious microstructure design. |
| 语种 | 英语 |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/38979]  |
| 专题 | 化学研究所_绿色印刷实验室 |
| 作者单位 | 1.Chinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China 2.Qingdao Univ Sci & Technol, Minist Educ, Key Lab Rubber Plast, Qingdao 266042, Peoples R China 3.Natl Ctr Nanosci & Technol China, CAS Key Lab Nanosyst & Hierarch Fabricat, Beijing 100190, Peoples R China 4.Univ Cincinnati, Coll Engn & Appl Sci, Dept Mech & Mat Engn, Mat Sci & Engn Program, Cincinnati, OH 45221 USA |
| 推荐引用方式 GB/T 7714 | Tan, Dongxing,Zhao, Jian,Gao, Caiyan,et al. Carbon Nanoparticle Hybrid Aerogels: 3D Double-Interconnected Network Porous Microstructure, Thermoelectric, and Solvent-Removal Functions[J]. ACS APPLIED MATERIALS & INTERFACES,2017,9(26):21820-21828. |
| APA | Tan, Dongxing,Zhao, Jian,Gao, Caiyan,Wang, Hanfu,Chen, Guangming,&Shi, Donglu.(2017).Carbon Nanoparticle Hybrid Aerogels: 3D Double-Interconnected Network Porous Microstructure, Thermoelectric, and Solvent-Removal Functions.ACS APPLIED MATERIALS & INTERFACES,9(26),21820-21828. |
| MLA | Tan, Dongxing,et al."Carbon Nanoparticle Hybrid Aerogels: 3D Double-Interconnected Network Porous Microstructure, Thermoelectric, and Solvent-Removal Functions".ACS APPLIED MATERIALS & INTERFACES 9.26(2017):21820-21828. |
入库方式： OAI收割
来源：化学研究所
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