Ultrathin and Ion-Selective Janus Membranes for High-Performance Osmotic Energy Conversion
文献类型:期刊论文
作者 | Zhang, Zhen1,4; Sui, Xin2; Li, Pei2; Xie, Ganhua1,4; Kong, Xiang-Yu3; Xiao, Kai1,4; Gao, Longcheng2; Wen, Liping2,3,4; Jiang, Lei2,3,4 |
刊名 | JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
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出版日期 | 2017-07-05 |
卷号 | 139期号:26页码:8905-8914 |
英文摘要 | The osmotic energy existing in fluids is recognized as a promising "blue" energy source that can help solve the global issues of energy shortage and environmental pollution. Recently, nanofluidic channels have shown great potential for capturing this worldwide energy because of their novel transport properties contributed by nanoconfinement. However, with respect to membrane-scale porous systems, high resistance and undesirable ion selectivity remain bottlenecks, impeding their applications. The development of thinner, low-resistance membranes, meanwhile promoting their ion selectivity, is a necessity. Here, we engineered ultrathin and ion-selective Janus membranes prepared via the phase separation,of two block copolymers, which enable osmotic energy conversion with power densities of approximately 2.04 W/m(2) by mixing natural seawater and river water. Both experiments and continuum simulation help us to understand the mechanism for how membrane thickness and channel structure dominate the ion transport process and overall device performance, which can serve as a general guiding principle for the future design of nanochannel membranes for high-energy concentration cells. |
语种 | 英语 |
源URL | [http://ir.iccas.ac.cn/handle/121111/39013] ![]() |
专题 | 化学研究所_绿色印刷实验室 |
作者单位 | 1.Chinese Acad Sci, Inst Chem, Key Lab Green Printing, BNLMS, Beijing 100190, Peoples R China 2.Beihang Univ, Sch Chem & Environm, Beijing 100191, Peoples R China 3.Chinese Acad Sci, Tech Inst Phys & Chem, Key Lab Bioinspired Mat & Interfacial Sci, Beijing 100190, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Zhen,Sui, Xin,Li, Pei,et al. Ultrathin and Ion-Selective Janus Membranes for High-Performance Osmotic Energy Conversion[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2017,139(26):8905-8914. |
APA | Zhang, Zhen.,Sui, Xin.,Li, Pei.,Xie, Ganhua.,Kong, Xiang-Yu.,...&Jiang, Lei.(2017).Ultrathin and Ion-Selective Janus Membranes for High-Performance Osmotic Energy Conversion.JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,139(26),8905-8914. |
MLA | Zhang, Zhen,et al."Ultrathin and Ion-Selective Janus Membranes for High-Performance Osmotic Energy Conversion".JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 139.26(2017):8905-8914. |
入库方式: OAI收割
来源:化学研究所
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