Shape-dependent ordering of gold nanocrystals into large-scale superlattices
文献类型：期刊论文
| 作者 | Gong, JX; Newman, RS; Engel, M; Zhao, M; Bian, FG; Glotzer, SC; Tang, ZY |
| 刊名 | NATURE COMMUNICATIONS
 |
| 出版日期 | 2017 |
| 卷号 | 8页码:- |
| ISSN号 | 2041-1723 |
| DOI | 10.1038/ncomms14038 |
| 文献子类 | 期刊论文 |
| 英文摘要 | Self-assembly of individual building blocks into highly ordered structures, analogous to spontaneous growth of crystals from atoms, is a promising approach to realize the collective properties of nanocrystals. Yet the ability to reliably produce macroscopic assemblies is unavailable and key factors determining assembly quality/yield are not understood. Here we report the formation of highly ordered superlattice films, with single crystalline domains of up to half a millimetre in two dimensions and thickness of up to several microns from nanocrystals with tens of nanometres in diameter. Combining experimental and computational results for gold nanocrystals in the shapes of spheres, cubes, octahedra and rhombic dodecahedra, we investigate the entire self-assembly process from disordered suspensions to large-scale ordered superlattices induced by nanocrystal sedimentation and eventual solvent evaporation. Our findings reveal that the ultimate coherence length of superlattices strongly depends on nanocrystal shape. Factors inhibiting the formation of high-quality large-scale superlattices are explored in detail. |
| 语种 | 英语 |
| WOS记录号 | WOS:000392178500001 |
| 源URL | [http://ir.sinap.ac.cn/handle/331007/27440]  |
| 专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
| 推荐引用方式 GB/T 7714 | Gong, JX,Newman, RS,Engel, M,et al. Shape-dependent ordering of gold nanocrystals into large-scale superlattices[J]. NATURE COMMUNICATIONS,2017,8:-. |
| APA | Gong, JX.,Newman, RS.,Engel, M.,Zhao, M.,Bian, FG.,...&Tang, ZY.(2017).Shape-dependent ordering of gold nanocrystals into large-scale superlattices.NATURE COMMUNICATIONS,8,-. |
| MLA | Gong, JX,et al."Shape-dependent ordering of gold nanocrystals into large-scale superlattices".NATURE COMMUNICATIONS 8(2017):-. |
入库方式： OAI收割
来源：上海应用物理研究所
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