Great Disparity in Photoluminesence Quantum Yields of Colloidal CsPbBr3 Nanocrystals with Varied Shape: The Effect of Crystal Lattice Strain
文献类型:期刊论文
作者 | Zhao, JT; Liu, M; Fang, L; Jiang, SL; Zhou, JT; Ding, HY; Huang, HW; Wen, W; Luo, ZL; Zhang, Q |
刊名 | JOURNAL OF PHYSICAL CHEMISTRY LETTERS
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出版日期 | 2017 |
卷号 | 8期号:13页码:3115-3121 |
关键词 | Cesium Lead Halide Perovskite Nanoplatelets Cdse Nanocrystals Dots Size Luminescent Growth Nanowires Emission Dynamics |
ISSN号 | 1948-7185 |
DOI | 10.1021/acs.jpclett.7b01083 |
文献子类 | 期刊论文 |
英文摘要 | Understanding the big discrepancy in the photoluminesence quantum yields (PLQYs) of nanoscale colloidal materials with varied morphologies is of great significance to its property optimization and functional application. Using different shaped CsPbBr3 nanocrystals with the same fabrication processes as model, quantitative synchrotron radiation X-ray diffraction analysis reveals the increasing trend in lattice strain values of the nanocrystals: nanocube, nanoplate, nanowire. Furthermore, transient spectroscopic measurements reveal the same trend in the defect quantities of these nanocrystals. These experimental results unambiguously point out that large lattice strain existing in CsPbBr3 nanoparticles induces more crystal defects and thus decreases the PLQY, implying that lattice strain is a key factor other than the surface defect to dominate the PLQY of colloidal photoluminesence materials. |
WOS关键词 | CESIUM LEAD HALIDE ; PEROVSKITE NANOPLATELETS ; CDSE NANOCRYSTALS ; DOTS ; SIZE ; LUMINESCENT ; GROWTH ; NANOWIRES ; EMISSION ; DYNAMICS |
语种 | 英语 |
WOS记录号 | WOS:000405252600053 |
源URL | [http://ir.sinap.ac.cn/handle/331007/28673] ![]() |
专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
推荐引用方式 GB/T 7714 | Zhao, JT,Liu, M,Fang, L,et al. Great Disparity in Photoluminesence Quantum Yields of Colloidal CsPbBr3 Nanocrystals with Varied Shape: The Effect of Crystal Lattice Strain[J]. JOURNAL OF PHYSICAL CHEMISTRY LETTERS,2017,8(13):3115-3121. |
APA | Zhao, JT.,Liu, M.,Fang, L.,Jiang, SL.,Zhou, JT.,...&Gao, C.(2017).Great Disparity in Photoluminesence Quantum Yields of Colloidal CsPbBr3 Nanocrystals with Varied Shape: The Effect of Crystal Lattice Strain.JOURNAL OF PHYSICAL CHEMISTRY LETTERS,8(13),3115-3121. |
MLA | Zhao, JT,et al."Great Disparity in Photoluminesence Quantum Yields of Colloidal CsPbBr3 Nanocrystals with Varied Shape: The Effect of Crystal Lattice Strain".JOURNAL OF PHYSICAL CHEMISTRY LETTERS 8.13(2017):3115-3121. |
入库方式: OAI收割
来源:上海应用物理研究所
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