Hydrophobic nanochannel self-assembled by amphipathic Janus particles confined in aqueous nano-space
文献类型：期刊论文
| 作者 | Fang, G; Sheng, N; Jin, T; Xu, YS; Sun, H; Yao, J; Zhuang, W; Fang, HP |
| 刊名 | CHINESE PHYSICS B
 |
| 出版日期 | 2018 |
| 卷号 | 27期号:3页码:- |
| 关键词 | Oil-water Interface Carbon Nanotubes Simulation Molecules Transport Channels Shale Nanoparticles Wettability Fabrication |
| ISSN号 | 1674-1056 |
| DOI | 10.1088/1674-1056/27/3/030505 |
| 文献子类 | 期刊论文 |
| 英文摘要 | Hydrophobic nanochannel plays a significant role in many physical, biological, and geological phenomena and exhibits impressive applications due to both its ubiquitous distribution and great ability to transport hydrophobic molecules, including various oils and gases. Based on theoretical modeling, we herein reveal that the amphipathic Janus nanoparticles have a large probability to self-assemble into uninterrupted hydrophobic nanochannels inside the aqueous nano-space, although there are large portions of the Janus nanoparticles to be hydrophilic. The key to this observation is the attractions between the hydrophobic regimes on neighboring amphipathic Janus particles through hydrophobic interaction in aqueous nano-space. More surprisingly, the permeation efficiency of hydrophobic molecules through the uninterrupted hydrophobic channel in Janus particles aggregate is even higher than that in the aggregate of hydrophobic particles. We note that the proposed amphipathic Janus particles can be transported to the appropriate positions by the water since the hydrophilic regimes still remain a strong particle-water interaction. We also note that most natural subsurface rocks are not completely hydrophobic or hydrophilic but have complex surfaces with inhomogeneous wetting property. Our work therefore provides a detailed molecular level understanding of the formation of underground strata as well as the new insight for constructing the artificial hydrophobic channels for various applications, such as the design of proppants to enhance the recovery of the unconventional oil/gas. |
| 语种 | 英语 |
| WOS记录号 | WOS:000428435600005 |
| 源URL | [http://ir.sinap.ac.cn/handle/331007/29034]  |
| 专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
| 作者单位 | 1.Fang, G 2.Sheng, N 3.Jin, T 4.Xu, YS 5.Sun, H 6.Yao, J 7.Zhuang, W 8.Fang, HP |
| 推荐引用方式 GB/T 7714 | Fang, G,Sheng, N,Jin, T,et al. Hydrophobic nanochannel self-assembled by amphipathic Janus particles confined in aqueous nano-space[J]. CHINESE PHYSICS B,2018,27(3):-. |
| APA | Fang, G.,Sheng, N.,Jin, T.,Xu, YS.,Sun, H.,...&Fang, HP.(2018).Hydrophobic nanochannel self-assembled by amphipathic Janus particles confined in aqueous nano-space.CHINESE PHYSICS B,27(3),-. |
| MLA | Fang, G,et al."Hydrophobic nanochannel self-assembled by amphipathic Janus particles confined in aqueous nano-space".CHINESE PHYSICS B 27.3(2018):-. |
入库方式： OAI收割
来源：上海应用物理研究所
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