In situ X-ray scattering observation of two-dimensional interfacial colloidal crystallization
文献类型:期刊论文
作者 | Wu, LL; Wang, X; Wang, G; Chen, G |
刊名 | NATURE COMMUNICATIONS
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出版日期 | 2018 |
卷号 | 9页码:- |
关键词 | Charged Particles Liquid Interfaces Electric-field Attraction Crystals |
ISSN号 | 2041-1723 |
DOI | 10.1038/s41467-018-03767-y |
文献子类 | 期刊论文 |
英文摘要 | Charged colloids at interfaces hold such a simple configuration that their interactions are supposed to be fully elucidated in the framework of classical electrostatics, yet the mysterious existence of attractive forces between these like-charged particles has puzzled the scientific community for decades. Here, we perform the in situ grazing-incidence small-angle X-ray scattering study of the dynamic self-assembling process of two-dimensional interfacial colloids. This approach allows simultaneous monitoring of the in-plane structure and ordering and the out-of-plane immersion depth variation. Upon compression, the system undergoes multiple metastable intermediate states before the stable hexagonal close-packed monolayer forms under van der Waals attraction. Remarkably, the immersion depth of colloidal particles is found to increase as the interparticle distance decreases. Numerical simulations demonstrate the interface around a colloid is deformed by the electrostatic force from its neighboring particles, which induces the long-range capillary attraction. |
语种 | 英语 |
WOS记录号 | WOS:000429399900008 |
源URL | [http://ir.sinap.ac.cn/handle/331007/29047] ![]() |
专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
作者单位 | 1.Wu, LL 2.Wang, X 3.Wang, G 4.Chen, G |
推荐引用方式 GB/T 7714 | Wu, LL,Wang, X,Wang, G,et al. In situ X-ray scattering observation of two-dimensional interfacial colloidal crystallization[J]. NATURE COMMUNICATIONS,2018,9:-. |
APA | Wu, LL,Wang, X,Wang, G,&Chen, G.(2018).In situ X-ray scattering observation of two-dimensional interfacial colloidal crystallization.NATURE COMMUNICATIONS,9,-. |
MLA | Wu, LL,et al."In situ X-ray scattering observation of two-dimensional interfacial colloidal crystallization".NATURE COMMUNICATIONS 9(2018):-. |
入库方式: OAI收割
来源:上海应用物理研究所
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