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Aluminum-Doped Cesium Lead Bromide Perovskite Nanocrystals with Stable Blue Photoluminescence Used for Display Backlight

文献类型:期刊论文

作者Ming Liu; Guo-Hua Zhong; Yongming Yin; Jingsheng Miao; Ke Li; Chengqun Wang; Xiuru Xu; Clifton Shen; Hong Meng
刊名Advanced Science
出版日期2017
文献子类期刊论文
英文摘要Bright and stable blue emitters with narrow full-width at half-maxima are particularly desirable for applications in television displays and related technologies. Here, this study shows that doping aluminum (Al3+) ion into CsPbBr3 nanocrystals (NCs) using AlBr3 can afford lead-halide perovskites NCs with stable blue photoluminescence. First, theoretical and experimental analyses reveal that the extended band gap and quantum confinement effect of elongated shape give rise to the desirable blueshifted emission. Second, the aluminum ion incorporation path is rationalized qualitatively by invoking fundamental considerations about binding relations in AlBr3 and its dimer. Finally, the absence of anion-exchange effect is corroborated when green CsPbBr3 and blue Al:CsPbBr3 NCs are mixed. Combinations of the above two NCs with red-emitting CdSe@ZnS NCs result in UV-pumped white lightemitting diodes (LED) with an National Television System Committee (NTSC) value of 116% and ITU-R Recommendation B.T. 2020 (Rec. 2020) of 87%. The color coordinates of the white LED are optimized at (0.32, 0.34) in CIE 1931. The results suggest that low-cost, earth-abundant, solution-processable Aldoped perovskite NCs can be promising candidate materials for blue downconversion layer in backlit displays.
URL标识查看原文
语种英语
WOS记录号WOS:000416155900019
源URL[http://ir.siat.ac.cn:8080/handle/172644/11613]  
专题深圳先进技术研究院_集成所
作者单位Advanced Science
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Ming Liu,Guo-Hua Zhong,Yongming Yin,et al. Aluminum-Doped Cesium Lead Bromide Perovskite Nanocrystals with Stable Blue Photoluminescence Used for Display Backlight[J]. Advanced Science,2017.
APA Ming Liu.,Guo-Hua Zhong.,Yongming Yin.,Jingsheng Miao.,Ke Li.,...&Hong Meng.(2017).Aluminum-Doped Cesium Lead Bromide Perovskite Nanocrystals with Stable Blue Photoluminescence Used for Display Backlight.Advanced Science.
MLA Ming Liu,et al."Aluminum-Doped Cesium Lead Bromide Perovskite Nanocrystals with Stable Blue Photoluminescence Used for Display Backlight".Advanced Science (2017).

入库方式: OAI收割

来源:深圳先进技术研究院

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