Femtosecond-laser-induced nonadiabatic alignment in photoexcited pyrimidine
文献类型：期刊论文
| 作者 | Jin, Bing; Zhang, Bing2; Ling, Fengzi; Li, Shuai; Wang, Yanmei; Long, Jinyou; Deng, Xulan |
| 刊名 | PHYSICAL REVIEW A
 |
| 出版日期 | 2017-09-29 |
| 卷号 | 96期号:3 |
| DOI | 10.1103/PhysRevA.96.033419 |
| 文献子类 | Article |
| 英文摘要 | The rotationalwave-packet dynamics in electronically excited pyrimidine induced by a femtosecond laser pulse at 321.5 nm has been studied by time-resolved mass spectroscopy and photoelectron velocity-map imaging. The rotational revival features at 81.3 ps, which are the direct manifestation of field-free nonadiabatic alignment, are clearly observed in both the time-dependent ion yields and photoelectron angular distributions. In particular, the out-of-phase recurrences in the parent-ion and fragment-ions transients indicate the different directions of the ionization transition-dipole moments for the generation of the parent ion and fragment ions. By tuning the polarization of the probe light parallel or perpendicular to that of the pump light, we demonstrate the potential application of nonadiabatic alignment to manipulate the branching ratio of photoionization products. |
| WOS关键词 | PHOTOELECTRON ANGULAR-DISTRIBUTIONS ; ALIGNED MOLECULES ; SPECTROSCOPY ; PHOTODISSOCIATION ; FIELDS ; DYNAMICS |
| WOS研究方向 | Optics ; Physics |
| 语种 | 英语 |
| WOS记录号 | WOS:000412026600008 |
| 资助机构 | National Basic Research Program of China (973 Program(2013CB922200) ; National Basic Research Program of China (973 Program(2013CB922200) ; National Natural Science Foundation of China(91121006 ; National Natural Science Foundation of China(91121006 ; 21327804 ; 21327804 ; 21573279 ; 21573279 ; 21303255 ; 21303255 ; Y6S0011037 ; Y6S0011037 ; 21503270 ; 21503270 ; 11674355 ; 11674355 ; 11574351) ; 11574351) ; National Basic Research Program of China (973 Program(2013CB922200) ; National Basic Research Program of China (973 Program(2013CB922200) ; National Natural Science Foundation of China(91121006 ; National Natural Science Foundation of China(91121006 ; 21327804 ; 21327804 ; 21573279 ; 21573279 ; 21303255 ; 21303255 ; Y6S0011037 ; Y6S0011037 ; 21503270 ; 21503270 ; 11674355 ; 11674355 ; 11574351) ; 11574351) |
| 源URL | [http://ir.wipm.ac.cn/handle/112942/11407]  |
| 专题 | 武汉物理与数学研究所_原子分子光物理研究部 |
| 作者单位 | 1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 2.Chinese Acad Sci, Wuhan Inst Phys & Math, State Key Lab Magnet Resonance & Atom & Mol Phys, Wuhan 430071, Hubei, Peoples R China |
| 推荐引用方式 GB/T 7714 | Jin, Bing,Zhang, Bing,Ling, Fengzi,et al. Femtosecond-laser-induced nonadiabatic alignment in photoexcited pyrimidine[J]. PHYSICAL REVIEW A,2017,96(3). |
| APA | Jin, Bing.,Zhang, Bing.,Ling, Fengzi.,Li, Shuai.,Wang, Yanmei.,...&Deng, Xulan.(2017).Femtosecond-laser-induced nonadiabatic alignment in photoexcited pyrimidine.PHYSICAL REVIEW A,96(3). |
| MLA | Jin, Bing,et al."Femtosecond-laser-induced nonadiabatic alignment in photoexcited pyrimidine".PHYSICAL REVIEW A 96.3(2017). |
入库方式： OAI收割
来源：武汉物理与数学研究所
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