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High Performance Solid Polymer Electrolytes for Rechargeable Batteries: A Self-Catalyzed Strategy toward Facile Synthesis

文献类型：期刊论文

作者Liu, Xiaochen1,4; Cui, Yanyan1,4; Liang, Xinmiao2,3; Chai, Jingchao1,2; Cui, Zili1,2; Wang, Qinglei1,2; He, Weisheng1,4; Liu, Zhihong1,2; Cui, Guanglei1,2; Feng, Jiwen2,3
刊名ADVANCED SCIENCE
出版日期2017-11-01
卷号4期号:11
关键词Cationic Mechanism Crosslinking In Situ Polymerization Poly(Ethylene Glycol) Diglycidyl Ether Solid Polymer Electrolytes
ISSN号2198-3844
DOI10.1002/advs.201700174
文献子类Article
英文摘要It is urgent to seek high performance solid polymer electrolytes (SPEs) via a facile chemistry and simple process. The lithium salts are composed of complex anions that are stabilized by a Lewis acid agent. This Lewis acid can initiate the ring opening polymerization. Herein, a self-catalyzed strategy toward facile synthesis of crosslinked poly(ethylene glycol) diglycidyl ether-based solid polymer electrolyte (C-PEGDE) is presented. It is manifested that the poly(ethylene glycol) diglycidyl ether-based solid polymer electrolyte possesses a superior electrochemical stability window up to 4.5 V versus Li/Li+ and considerable ionic conductivity of 8.9 x 10(-5) S cm(-1) at ambient temperature. Moreover, the LiFePO4/C-PEGDE/Li batteries deliver stable charge/discharge profiles and considerable rate capability. It is demonstrated that this self-catalyzed strategy can be a very effective approach for high performance solid polymer electrolytes.
WOS关键词LITHIUM-ION BATTERIES ; POLY(ETHYLENE OXIDE) ; ROOM-TEMPERATURE ; CONDUCTIVITY ; LIQUID ; REINFORCEMENT ; COPOLYMERS ; TRANSPORT ; CELLULOSE ; MEMBRANE
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science
语种英语
WOS记录号WOS:000416155900011
出版者WILEY
资助机构Chinese Academy of Sciences(XDA09010105) ; Chinese Academy of Sciences(XDA09010105) ; Shandong Provincial Natural Science Foundation, China(ZR2015QZ01) ; Shandong Provincial Natural Science Foundation, China(ZR2015QZ01) ; CAS-QIBEBT Director Innovation Foundation ; CAS-QIBEBT Director Innovation Foundation ; Qingdao Key Lab of solar energy utilization and energy storage technology ; Qingdao Key Lab of solar energy utilization and energy storage technology ; Chinese Academy of Sciences(XDA09010105) ; Chinese Academy of Sciences(XDA09010105) ; Shandong Provincial Natural Science Foundation, China(ZR2015QZ01) ; Shandong Provincial Natural Science Foundation, China(ZR2015QZ01) ; CAS-QIBEBT Director Innovation Foundation ; CAS-QIBEBT Director Innovation Foundation ; Qingdao Key Lab of solar energy utilization and energy storage technology ; Qingdao Key Lab of solar energy utilization and energy storage technology ; Chinese Academy of Sciences(XDA09010105) ; Chinese Academy of Sciences(XDA09010105) ; Shandong Provincial Natural Science Foundation, China(ZR2015QZ01) ; Shandong Provincial Natural Science Foundation, China(ZR2015QZ01) ; CAS-QIBEBT Director Innovation Foundation ; CAS-QIBEBT Director Innovation Foundation ; Qingdao Key Lab of solar energy utilization and energy storage technology ; Qingdao Key Lab of solar energy utilization and energy storage technology ; Chinese Academy of Sciences(XDA09010105) ; Chinese Academy of Sciences(XDA09010105) ; Shandong Provincial Natural Science Foundation, China(ZR2015QZ01) ; Shandong Provincial Natural Science Foundation, China(ZR2015QZ01) ; CAS-QIBEBT Director Innovation Foundation ; CAS-QIBEBT Director Innovation Foundation ; Qingdao Key Lab of solar energy utilization and energy storage technology ; Qingdao Key Lab of solar energy utilization and energy storage technology
源URL[http://ir.wipm.ac.cn/handle/112942/12730]  
专题中国科学院武汉物理与数学研究所
通讯作者Liu, Zhihong; Cui, Guanglei
作者单位1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao Ind Energy Storage Res Inst, Qingdao 266101, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Wuhan Inst Phys & Math, State Key Lab Magnet Resonance & Atom & Mol Phys, Wuhan 430071, Hubei, Peoples R China
4.Qingdao Univ Sci & Technol, Key Lab Nanomat, Qingdao 266042, Peoples R China
推荐引用方式
GB/T 7714		 Liu, Xiaochen,Cui, Yanyan,Liang, Xinmiao,et al. High Performance Solid Polymer Electrolytes for Rechargeable Batteries: A Self-Catalyzed Strategy toward Facile Synthesis[J]. ADVANCED SCIENCE,2017,4(11).
APA Liu, Xiaochen.,Cui, Yanyan.,Liang, Xinmiao.,Chai, Jingchao.,Cui, Zili.,...&Feng, Jiwen.(2017).High Performance Solid Polymer Electrolytes for Rechargeable Batteries: A Self-Catalyzed Strategy toward Facile Synthesis.ADVANCED SCIENCE,4(11).
MLA Liu, Xiaochen,et al."High Performance Solid Polymer Electrolytes for Rechargeable Batteries: A Self-Catalyzed Strategy toward Facile Synthesis".ADVANCED SCIENCE 4.11(2017).

入库方式： OAI收割

来源：武汉物理与数学研究所

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