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Influence of pyroxene and spinel on the kinetics of peridotite serpentinization

文献类型：期刊论文

作者Huang, Ruifang1,2; Song, Maoshuang3; Ding, Xing3; Zhu, Sanyuan4; Zhan, Wenhuan2; Sun, Weidong5,6,7
刊名JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH
出版日期2017-09-01
卷号122期号:9页码:7111-7126
关键词Serpentinization Kinetics Peridotite Spinel Aluminum Chromium
ISSN号2169-9313
DOI10.1002/2017JB014231
文献子类Article
英文摘要Hydrothermal experiments were performed at 311 degrees C and 3.0 kbar on natural olivine and peridotite to investigate the kinetics of serpentinization. The results show that the rates of reaction strongly depend on grain sizes of solid reactants, with smaller grain sizes resulting in faster kinetics. After 27 days of reaction, the reaction extent was 99% for peridotite with grain sizes of <30 mu m, and the reaction extent was 28% for grain sizes of 100-177 mu m. Compared to peridotite, olivine is serpentinized at much slower rates, e.g., 5.3% of reaction extent was achieved for olivine with grain sizes of 100-177 mu m after 27 days, approximately five times lower than that reached during peridotite serpentinization. Such contrasting results are due to the presence of pyroxene and spinel, an interpretation which is supported by a marked increase in reaction extents for experiments with the addition of pyroxene and spinel. The reaction extent achieved in experiments with 3 wt% spinel greatly increased to 98% after 27 days, much higher than that achieved during olivine serpentinization. These results appear to be related to pyroxene and spinel releasing Al and Cr during serpentinization. As indicated by compositions of serpentine, orthopyroxene lost similar to 60% of Al at a reaction extent of 59%. Influence of Al and Cr is suggested by a dramatic increase in reaction extents with the addition of Al2O3 and Cr2O3 powders. Olivine in natural geological settings is commonly associated with pyroxene and spinel; consequently, serpentinization kinetics may be much faster than previously thought.
WOS关键词MID-ATLANTIC RIDGE ; HOSTED HYDROTHERMAL SYSTEMS ; FORE-ARC MANTLE ; VENT FLUIDS ; LOST CITY ; CHEMICAL-COMPOSITION ; ABYSSAL PERIDOTITES ; HYDRATION REACTIONS ; ULTRAMAFIC ROCKS ; MIDOCEAN RIDGES
WOS研究方向Geochemistry & Geophysics
语种英语
WOS记录号WOS:000412881700009
出版者AMER GEOPHYSICAL UNION
资助机构Natural Science Foundation of China(41603060 ; China postdoctoral Science Foundation(2015M570735 ; Chinese Academy of Sciences(XDB06030100) ; 91328204) ; 2016T90805)
源URL[http://ir.qibebt.ac.cn/handle/337004/10461]  
专题中国科学院青岛生物能源与过程研究所
通讯作者Huang, Ruifang; Sun, Weidong
作者单位1.Chinese Acad Sci, Guangzhou Inst Geochem, Key Lab Mineral & Metallogeny, Guangzhou, Guangdong, Peoples R China
2.Chinese Acad Sci, South China Sea Inst Oceanol, Key Lab Ocean & Marginal Sea Geol, Guangzhou, Guangdong, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Isotope Geochem, Guangzhou, Guangdong, Peoples R China
4.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou, Guangdong, Peoples R China
5.Chinese Acad Sci, Inst Oceanol, Ctr Deep Sea Res, Qingdao, Peoples R China
6.Qingdao Natl Lab Marine Sci & Technol, Lab Marine Mineral Resources, Qingdao, Peoples R China
7.Chinese Acad Sci, CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing, Peoples R China
推荐引用方式
GB/T 7714		 Huang, Ruifang,Song, Maoshuang,Ding, Xing,et al. Influence of pyroxene and spinel on the kinetics of peridotite serpentinization[J]. JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH,2017,122(9):7111-7126.
APA Huang, Ruifang,Song, Maoshuang,Ding, Xing,Zhu, Sanyuan,Zhan, Wenhuan,&Sun, Weidong.(2017).Influence of pyroxene and spinel on the kinetics of peridotite serpentinization.JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH,122(9),7111-7126.
MLA Huang, Ruifang,et al."Influence of pyroxene and spinel on the kinetics of peridotite serpentinization".JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH 122.9(2017):7111-7126.

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来源：青岛生物能源与过程研究所

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