中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Carbon Dioxide Sequestration via Steelmaking Slag Carbonation in Alkali Solutions: Experimental Investigation and Process Evaluation

文献类型:期刊论文

作者Wang, Chen-Ye1,2; Bao, Wei-Jun2; Guo, Zhan-Cheng1; Li, Hui-Quan2
刊名ACTA METALLURGICA SINICA-ENGLISH LETTERS
出版日期2018-07-01
卷号31期号:7页码:771-784
关键词Steelmaking Slag Dilute Alkali Solution Co2 Mineral Sequestration Process Evaluation
ISSN号1006-7191
DOI10.1007/s40195-017-0694-0
英文摘要

Carbon dioxide mineral sequestration with steelmaking slag is a promising method for reducing carbon dioxide in a largescale setting. Existing calcium oxide or calcium hydroxide in steelmaking slag can be easily leached by water, and the formed calcium carbonate can be easily wrapped on the surface of unreacted steelmaking slag particles. Thus, further increase in the carbonation reaction rate can be prevented. Enhanced carbon dioxide mineral sequestration with steelmaking slag in dilute alkali solution was analysed in this study through experiments and process evaluation. Operating conditions, namely alkali concentration, reaction temperature and time, and liquid-to-solid ratio, were initially investigated. Then, the material and energy balance of the entire process was calculated, and the net carbon dioxide sequestration efficiency at different reaction times was evaluated. Results showed that dilute alkali solution participated in slowing down the leaching of active calcium in the steelmaking slag and in significantly improving carbonation conversion rate. The highest carbonation conversion rate of approximately 50% can be obtained at the optimal conditions of 20 g/L alkali concentration, 2 mL/L liquid-to-solid ratio, and 70 degrees C reaction temperature. Carbonation reaction time significantly influences the net carbon dioxide sequestration efficiency. According to calculation, carbon dioxide emission of 52.6 kg/tslag was avoided at a relatively long time of 120 min.

WOS关键词Co2 Mineral Sequestration ; Precipitated Calcium-carbonate ; Steel Converter Slag ; Flue-gas Emissions ; Energy-consumption ; Capture
资助项目National Natural Science Foundation of China[21300212]
WOS研究方向Metallurgy & Metallurgical Engineering
语种英语
WOS记录号WOS:000433167400012
出版者CHINESE ACAD SCIENCES, INST METAL RESEARCH
资助机构National Natural Science Foundation of China
源URL[http://ir.ipe.ac.cn/handle/122111/24637]  
专题中国科学院过程工程研究所
通讯作者Li, Hui-Quan
作者单位1.Univ Sci & Technol Beijing, State Key Lab Adv Met, Beijing 100083, Peoples R China
2.Chinese Acad Sci, Natl Engn Lab Hydromet Cleaner Prod Technol, Key Lab Green Proc & Engn, Inst Proc Engn, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714
Wang, Chen-Ye,Bao, Wei-Jun,Guo, Zhan-Cheng,et al. Carbon Dioxide Sequestration via Steelmaking Slag Carbonation in Alkali Solutions: Experimental Investigation and Process Evaluation[J]. ACTA METALLURGICA SINICA-ENGLISH LETTERS,2018,31(7):771-784.
APA Wang, Chen-Ye,Bao, Wei-Jun,Guo, Zhan-Cheng,&Li, Hui-Quan.(2018).Carbon Dioxide Sequestration via Steelmaking Slag Carbonation in Alkali Solutions: Experimental Investigation and Process Evaluation.ACTA METALLURGICA SINICA-ENGLISH LETTERS,31(7),771-784.
MLA Wang, Chen-Ye,et al."Carbon Dioxide Sequestration via Steelmaking Slag Carbonation in Alkali Solutions: Experimental Investigation and Process Evaluation".ACTA METALLURGICA SINICA-ENGLISH LETTERS 31.7(2018):771-784.

入库方式: OAI收割

来源:过程工程研究所

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