Pyrolysis of Huadian Oil Shale in an Infrared Heating Reactor
文献类型:期刊论文
作者 | Siramard, Somprasong1,2; Bumnan, Yutthasin1,2; Lai, Dengguo1,2; Xu, Guangwen1 |
刊名 | ENERGY & FUELS
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出版日期 | 2017-07-01 |
卷号 | 31期号:7页码:6996-7003 |
ISSN号 | 0887-0624 |
DOI | 10.1021/acs.energyfuels.7b00964 |
文献子类 | Article |
英文摘要 | Pyrolysis of Huadian oil shale was investigated in a newly designed shallow fixed bed reactor mounted with infrared heating to clarify the pyrolysis behavior at different heating rates and pyrolysis temperatures under minimized secondary reactions to volatiles in an oil shale bed. The maximum shale oil recovery was obtained under the proper conditions of a heating rate of 0.5 degrees C/s, a pyrolysis temperature of about 550 degrees C, a reduced reaction pressure (0.6 atm in this work), and for a single layer oil shale bed. The highest shale oil yield under such conditions was close to 100% of the Fischer Assay oil yield (11.10 wt % of dry basis). For the adopted infrared-heating reactor, increasing the heating, rate decreased the shale oil yield but increased the gas production. The total hydrogen in volatile products including shale oil and pyrolysis gas increased with raising the heating rate, and the total volatile production was higher for the infrared quick heating pyrolysis (heating rate: 25 degrees C/s) than that for the Fischer Assay. The shale oil from the infrared quick heating pyrolysis had also more light fraction. Experiment also found that pyrolyzing the multilayer oil shale bed lowered the shale oil yield in comparison with the pyrolysis of a single-layer material bed. Thus, adopting a single-layer oil shale bed, low infrared heating rates, and reduced reaction pressures obviously suppressed the secondary reactions toward volatiles to have consequently high shale oil yield. High infrared heating rate facilitated volatile and hydrogen production but led to more serious secondary reactions to lower the shale oil yield. |
WOS关键词 | Rapid Pyrolysis ; Products Yield ; Particle-size ; Grain-size ; Fixed-bed ; Coal ; Evolution ; Catalyst ; Goynuk |
WOS研究方向 | Energy & Fuels ; Engineering |
语种 | 英语 |
WOS记录号 | WOS:000406356600034 |
资助机构 | National Basic Research Program of China(2014CB744303) ; National Natural Science Foundation(91534125) ; CAS-TWAS |
源URL | [http://ir.ipe.ac.cn/handle/122111/23172] ![]() |
专题 | 过程工程研究所_多相复杂系统国家重点实验室 |
作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Siramard, Somprasong,Bumnan, Yutthasin,Lai, Dengguo,et al. Pyrolysis of Huadian Oil Shale in an Infrared Heating Reactor[J]. ENERGY & FUELS,2017,31(7):6996-7003. |
APA | Siramard, Somprasong,Bumnan, Yutthasin,Lai, Dengguo,&Xu, Guangwen.(2017).Pyrolysis of Huadian Oil Shale in an Infrared Heating Reactor.ENERGY & FUELS,31(7),6996-7003. |
MLA | Siramard, Somprasong,et al."Pyrolysis of Huadian Oil Shale in an Infrared Heating Reactor".ENERGY & FUELS 31.7(2017):6996-7003. |
入库方式: OAI收割
来源:过程工程研究所
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