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Design Synthesis of ITE Zeolite Using Nickel-Amine Complex as an Efficient Structure-Directing Agent

文献类型：期刊论文

作者Xiao, Feng-Shou4; Meng, Xiangju4; Jin, Chuanhong1; Zheng, Anmin2; Zhu, Longfeng3,4; Wang, Liang4; Zhang, Jian4; Chen, Wei2; Wu, Qinming1,4; Han, Shichao4
刊名ACS APPLIED MATERIALS & INTERFACES
出版日期2018-10-03
卷号10期号:39页码:33214-33220
关键词zeolite ITE nickel-pentaethylenexamine design synthesis hydrogenation of CO2
ISSN号1944-8244
DOI10.1021/acsami.8b10620
英文摘要Modern methodologies for synthesizing zeolites typically involve the employment of costly organic structure-directing agents. Herein, we report the design synthesis of aluminosilicate zeolite with ITE structure using an inexpensive nickel amine complex (nickel-pentaethylenexamine) as a novel structure-directing agent. Characterizations including X-ray diffraction, scanning electron microscopy, N-2 sorption isotherms, and Al-27 magic-angle spinning NMR techniques show that the ITE zeolite has high crystallinity, perfect crystals, large surface area, and abundant aluminum species in the framework. More importantly, catalytic tests on the hydrogenation of CO2 into methane show that the Ni-ITE zeolite exhibits better catalytic performance than aluminosilicate-supported and silica-supported nickel catalysts. Obviously, the use of nickel amine complex offers an alternative and facile way to synthesize aluminosilicate zeolites.
WOS关键词SELECTIVE CATALYTIC-REDUCTION ; CARBON-DIOXIDE METHANATION ; ONE-POT SYNTHESIS ; CRYSTAL-STRUCTURE ; ACTIVE CATALYST ; FRAMEWORK ; TEMPLATE ; SILICA ; NANOPARTICLES ; STA-7
资助项目National Key Research and Development Program of China[2017YFB0702803] ; National Natural Science Foundation of China[91634201] ; National Natural Science Foundation of China[91545111] ; National Natural Science Foundation of China[21703203] ; National Natural Science Foundation of China[21802053] ; National Natural Science Foundation of China[21720102001] ; China Postdoctoral Science Foundation[2017M611978]
WOS研究方向Science & Technology - Other Topics ; Materials Science
语种英语
WOS记录号WOS:000446919800031
出版者AMER CHEMICAL SOC
资助机构National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation
源URL[http://ir.wipm.ac.cn/handle/112942/13305]  
专题武汉物理与数学研究所_磁共振应用研究部
通讯作者Meng, Xiangju; Wu, Qinming
作者单位1.Zhejiang Univ, Sch Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310007, Zhejiang, Peoples R China
2.Wuhan Inst Phys & Math, Wuhan Ctr Magnet Resonance, State Key Lab Magnet Resonance & Atom & Mol Phys, Wuhan 430071, Hubei, Peoples R China
3.Jiaxing Univ, Coll Biol Chem Sci & Engn, Jiaxing 314001, Peoples R China
4.Zhejiang Univ, Key Lab Appl Chem Zhejiang Prov, Hangzhou 310028, Zhejiang, Peoples R China
推荐引用方式
GB/T 7714		 Xiao, Feng-Shou,Meng, Xiangju,Jin, Chuanhong,et al. Design Synthesis of ITE Zeolite Using Nickel-Amine Complex as an Efficient Structure-Directing Agent[J]. ACS APPLIED MATERIALS & INTERFACES,2018,10(39):33214-33220.
APA Xiao, Feng-Shou.,Meng, Xiangju.,Jin, Chuanhong.,Zheng, Anmin.,Zhu, Longfeng.,...&Han, Shichao.(2018).Design Synthesis of ITE Zeolite Using Nickel-Amine Complex as an Efficient Structure-Directing Agent.ACS APPLIED MATERIALS & INTERFACES,10(39),33214-33220.
MLA Xiao, Feng-Shou,et al."Design Synthesis of ITE Zeolite Using Nickel-Amine Complex as an Efficient Structure-Directing Agent".ACS APPLIED MATERIALS & INTERFACES 10.39(2018):33214-33220.

入库方式： OAI收割

来源：武汉物理与数学研究所

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