Nitrogen-rich core-shell structured particles consisting of carbonized zeolitic imidazolate frameworks and reduced graphene oxide for amperometric determination of hydrogen peroxide
文献类型：期刊论文
| 作者 | Li, Zehui1; Jiang, Yuheng2; Wang, Zhuoya3; Wang, Wenbo4; Yuan, Yi3; Wu, Xiaoxue1; Liu, Xingchen1; Li, Mingjie5 ; Dilpazir, Sobia4; Zhang, Guangjin4
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| 刊名 | MICROCHIMICA ACTA
 |
| 出版日期 | 2018-11-01 |
| 卷号 | 185期号:11页码:9 |
| 关键词 | Electrochemical sensor Electrocatalyst Nitrogen doped carbon H2O2 Screen-printed electrode |
| ISSN号 | 0026-3672 |
| DOI | 10.1007/s00604-018-3032-y |
| 英文摘要 | Core-shell structured particles were prepared from carbonized zeolitic imidazolate frameworks (ZIFs) and reduced graphene oxide (rGO). The particles possess a nitrogen content of up to 10.6%. The loss of nitrogen from the ZIF is avoided by utilizing the reduction and agglomeration of graphene oxide with suitable size (>2 mu m) during pyrolysis. The resulting carbonized ZIF@rGO particles were deposited on a glassy carbon electrode to give an amperometric sensor for H2O2, typically operated at a voltage of -0.4V (vs. Ag/AgCl). The sensor has a wide detection range (from 5 x 10(-6) to 2 x 10(-2) M), a 3.3 mu M (S/N = 3) detection limit and a 0.272 mu A.mu M(-1.)cm(-2) sensitivity, much higher than that of directly carbonized ZIFs. The sensor material was also deposited on a screen-printed electrode to explore the possibility of application. |
| WOS关键词 | DOPED POROUS CARBON ; OXYGEN REDUCTION ; ELECTROCHEMICAL DETECTION ; NANOPARTICLE ; PERFORMANCE ; ELECTRODES ; EFFICIENT ; COMPOSITE ; SENSORS ; CELLS |
| 资助项目 | National Key R&D Program of China[2016YFC0200102] ; National Natural Science Foundation of China[91643201] ; National Natural Science Foundation of China[51608509] ; National Natural Science Foundation of China[91545125] ; National Natural Science Foundation of China[U1662121] ; Tsinghua Qingfeng Scholarship[THQF2018-16] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000446885200002 |
| 出版者 | SPRINGER WIEN |
| 资助机构 | National Key R&D Program of China ; National Natural Science Foundation of China ; Tsinghua Qingfeng Scholarship |
| 源URL | [http://ir.qibebt.ac.cn/handle/337004/11748]  |
| 专题 | 中国科学院青岛生物能源与过程研究所 |
| 通讯作者 | Jiang, Jingkun |
| 作者单位 | 1.Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China 2.Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China 3.China Univ Min & Technol, Sch Chem & Environm Engn, Beijing 100083, Peoples R China 4.Chinese Acad Sci, Beijing Engn Res Ctr Proc Pollut Control, Inst Proc Engn, Div Environm Technol & Engn, Beijing 100049, Peoples R China 5.Chinese Acad Sci, Qingdao Inst Biomass Energy & Bioproc Technol, Qingdao 266101, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Zehui,Jiang, Yuheng,Wang, Zhuoya,et al. Nitrogen-rich core-shell structured particles consisting of carbonized zeolitic imidazolate frameworks and reduced graphene oxide for amperometric determination of hydrogen peroxide[J]. MICROCHIMICA ACTA,2018,185(11):9. |
| APA | Li, Zehui.,Jiang, Yuheng.,Wang, Zhuoya.,Wang, Wenbo.,Yuan, Yi.,...&Jiang, Jingkun.(2018).Nitrogen-rich core-shell structured particles consisting of carbonized zeolitic imidazolate frameworks and reduced graphene oxide for amperometric determination of hydrogen peroxide.MICROCHIMICA ACTA,185(11),9. |
| MLA | Li, Zehui,et al."Nitrogen-rich core-shell structured particles consisting of carbonized zeolitic imidazolate frameworks and reduced graphene oxide for amperometric determination of hydrogen peroxide".MICROCHIMICA ACTA 185.11(2018):9. |
入库方式： OAI收割
来源：青岛生物能源与过程研究所
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