MAPbCI(3)-Mediated Decomposition Process to Tune Cl/Pbl(2) Distribution in MAPbl(3) Films
文献类型：期刊论文
| 作者 | Zhang, Cuiping1,2; Li, Zhipeng1,2; Liu, Juan2; Xin, Yunchuan1; Shao, Zhipeng1; Cui, Guanglei1 ; Pang, Shuping1
|
| 刊名 | ACS ENERGY LETTERS
 |
| 出版日期 | 2018-08-01 |
| 卷号 | 3期号:8页码:1801-1807 |
| ISSN号 | 2380-8195 |
| DOI | 10.1021/acsenergylett.8b00837 |
| 英文摘要 | Various methods have been developed to optimize the active layer of perovskite solar cells. To date, the introduction of excess PM, and chlorine doping are two typical means. Herein, an ion exchange decomposition process was designed to combine these two approaches. In this process, the I-Cl exchange and MACI sublimation occurred simultaneously at elevated temperature, resulting in a Pbl(2)-excess, Cl-doped perovskite film. This combined strategy could guarantee that as much chlorine as possible was doped into the perovskite crystal lattice, which enables the production of perovskite films with obviously reduced defect density and enhanced carrier diffusion length. Strikingly, the power conversion efficiency of the device is boosted from 17.17% to 20.15%. |
| WOS关键词 | PEROVSKITE SOLAR-CELLS ; METHYLAMMONIUM LEAD TRIIODIDE ; THIN-FILMS ; HALIDE PEROVSKITE ; CATION-EXCHANGE ; EFFICIENT ; PERFORMANCE ; EVOLUTION ; FORMAMIDINIUM ; TRIHALIDE |
| 资助项目 | National Natural Science Foundation of China[51672290] ; National Natural Science Foundation of China[21671196] ; Outstanding Youth Foundation of Shandong Province[JQ201813] ; DICPQIBEBT[UN201705] ; Youth Innovation Promotion Association of CAS[2015167] ; Qingdao Key Lab of Solar Energy Utilization and Energy Storage Technology |
| WOS研究方向 | Chemistry ; Electrochemistry ; Energy & Fuels ; Science & Technology - Other Topics ; Materials Science |
| 语种 | 英语 |
| WOS记录号 | WOS:000441852800004 |
| 出版者 | AMER CHEMICAL SOC |
| 资助机构 | National Natural Science Foundation of China ; Outstanding Youth Foundation of Shandong Province ; DICPQIBEBT ; Youth Innovation Promotion Association of CAS ; Qingdao Key Lab of Solar Energy Utilization and Energy Storage Technology |
| 源URL | [http://ir.qibebt.ac.cn/handle/337004/12157]  |
| 专题 | 中国科学院青岛生物能源与过程研究所 |
| 通讯作者 | Liu, Juan; Pang, Shuping |
| 作者单位 | 1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China 2.Qingdao Univ Sci & Technol, Qingdao 266042, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhang, Cuiping,Li, Zhipeng,Liu, Juan,et al. MAPbCI(3)-Mediated Decomposition Process to Tune Cl/Pbl(2) Distribution in MAPbl(3) Films[J]. ACS ENERGY LETTERS,2018,3(8):1801-1807. |
| APA | Zhang, Cuiping.,Li, Zhipeng.,Liu, Juan.,Xin, Yunchuan.,Shao, Zhipeng.,...&Pang, Shuping.(2018).MAPbCI(3)-Mediated Decomposition Process to Tune Cl/Pbl(2) Distribution in MAPbl(3) Films.ACS ENERGY LETTERS,3(8),1801-1807. |
| MLA | Zhang, Cuiping,et al."MAPbCI(3)-Mediated Decomposition Process to Tune Cl/Pbl(2) Distribution in MAPbl(3) Films".ACS ENERGY LETTERS 3.8(2018):1801-1807. |
入库方式： OAI收割
来源：青岛生物能源与过程研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。