中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
The extremely narrow hysteresis width of phase transition in nanocrystalline VO2 thin films with the flake grain structures

文献类型:期刊论文

作者Xu, XF; He, XF; Wang, HY; Gu, QJ; Shi, SX; Xing, HZ; Wang, CR; Zhang, J; Chen, XS; Chu, JH
刊名APPLIED SURFACE SCIENCE
出版日期2012
卷号261期号:0
英文摘要The nanocrystalline VO2 thin films, which surface has a flake grain structure, are achieved by DC sputtering deposition at different sputtering powers. It is found that the hysteresis loop of metal-insulator phase transition (MIT) is almost superposition, and the hysteresis width is only 0.4 degrees C for the surface flake grain structure that obtained at 132 W DC sputtering power. Moreover, it is shown that the phase transition is very steep, and the film displays 3-4 orders of the change of sheet resistance at MIT. The characterizations of SEM, AFM and four-point probe methods show that the hysteresis width, the orders of the change of sheet resistance and the phase transition become narrower, higher and steeper at MIT, respectively when the surface shapes of the nanocrystalline VO2 thin films change from nanoparticle structures to flake structures with the DC sputtering powers increased from 66 W to 132 W and the surface flake grain sizes reduced gradually to minimum at 132 W. Meanwhile, the surface roughness also changes into minimum. However, with the powers further increased from 132 W to 176 W, the surface flake grain sizes become bigger, and then the surface roughness changes poor. At 176 W, the surface flake structures begin to turn into nanoparticle structures. The hysteresis width, the orders of the change of sheet resistance and the phase transition become wider, lower and poorly steeper at MIT, separately. The results reveal that the nanocrystalline shapes and the surface roughness can affect the hysteresis width and the sheet resistance steepness in MIT. Our analysis shows that the mechanism of the narrowed hysteresis width mainly depends on the strain imbalance of the nanocrystalline VO2 thin film of the flake structures at MIT. (C) 2012 Elsevier B.V. All rights reserved.
WOS记录号WOS:000310442500013
公开日期2013-03-18
源URL[http://202.127.1.142/handle/181331/6941]  
专题上海技术物理研究所_上海技物所
推荐引用方式
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Xu, XF,He, XF,Wang, HY,et al. The extremely narrow hysteresis width of phase transition in nanocrystalline VO2 thin films with the flake grain structures[J]. APPLIED SURFACE SCIENCE,2012,261(0).
APA Xu, XF.,He, XF.,Wang, HY.,Gu, QJ.,Shi, SX.,...&Chu, JH.(2012).The extremely narrow hysteresis width of phase transition in nanocrystalline VO2 thin films with the flake grain structures.APPLIED SURFACE SCIENCE,261(0).
MLA Xu, XF,et al."The extremely narrow hysteresis width of phase transition in nanocrystalline VO2 thin films with the flake grain structures".APPLIED SURFACE SCIENCE 261.0(2012).

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来源:上海技术物理研究所

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