中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Different temperature dependence of excitonic and defect-related photoluminescence spectra in ZnS nanobelts and nanowires

文献类型:期刊论文

作者Wang, HY; Wang, CR; Xu, J; Liu, X; Xu, XF; Xing, HZ; Zhao, LJ; Chen, XS
刊名JOURNAL OF PHYSICS D-APPLIED PHYSICS
出版日期2012
卷号45期号:9
英文摘要In this paper, both excitonic and defect-related information of ZnS nanobelts and nanowires have been investigated by a temperature-dependent photoluminescence (PL) spectrum. PL spectra of ZnS nanobelts and nanowires differ significantly in the ultraviolet (UV) and visible emission regions. In UV emission regions, due to high-quality crystals, free exciton B (FXB), free exciton A (FXA), FXA-one longitudinal optical (LO) phonon replica are observed in ZnS nanobelts, as well as free-to-bound (e, A) with its one LO phonon replica, while neutral-donor bound exciton (D-o, X) and free-to-bound (e, A) are observed in ZnS nanowires at 10 K. The peak and relative intensity of the FX and (D-o, X) versus temperature follow well with conventional empirical relations. In the visible emission regions, weak donor-acceptor pair (DAP) and self-activated (SA) emission from ZnS nanowires are commonly observed, but the Y band emission is only observed at 10K in ZnS nanobelts. The Y band emission disappears at some temperature lower than 50 K. The peak position and full width at half maximum of DAP and SA emission bands display different temperature dependences. Detailed study on temperature-dependent PL spectra of ZnS nanobelts and nanowires provides crucial information on the nature of the electronic states and recombination mechanisms in these nanostructures.
WOS记录号WOS:000300773900007
公开日期2013-03-18
源URL[http://202.127.1.142/handle/181331/7113]  
专题上海技术物理研究所_上海技物所
推荐引用方式
GB/T 7714
Wang, HY,Wang, CR,Xu, J,et al. Different temperature dependence of excitonic and defect-related photoluminescence spectra in ZnS nanobelts and nanowires[J]. JOURNAL OF PHYSICS D-APPLIED PHYSICS,2012,45(9).
APA Wang, HY.,Wang, CR.,Xu, J.,Liu, X.,Xu, XF.,...&Chen, XS.(2012).Different temperature dependence of excitonic and defect-related photoluminescence spectra in ZnS nanobelts and nanowires.JOURNAL OF PHYSICS D-APPLIED PHYSICS,45(9).
MLA Wang, HY,et al."Different temperature dependence of excitonic and defect-related photoluminescence spectra in ZnS nanobelts and nanowires".JOURNAL OF PHYSICS D-APPLIED PHYSICS 45.9(2012).

入库方式: OAI收割

来源:上海技术物理研究所

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