Catalytic reduction of low-concentration CO2 with water by Pt/Co@NC
文献类型:期刊论文
作者 | Wang, Qianqian1,2; Wang, Wenzhong2; Zhang, Ling2; Su, Yang2; Wang, Kefu2; Wu, Huixia1 |
刊名 | JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
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出版日期 | 2018 |
卷号 | 34期号:12页码:2337 |
关键词 | Carbon dioxide catalytic reduction Pt/Co@NC Low-concentration CO2 No sacrificial agent |
ISSN号 | 1005-0302 |
DOI | 10.1016/j.jmst.2018.04.010 |
英文摘要 | The reduction of low-concentration carbon dioxide with water to organic fuels is still a huge challenge. In this study, we successfully designed the partially oxidized cobalt nanoparticles coated by the nitrogen-doped carbon layer (Co@NC) of 2-8 nm via a facile method and then interspersed with different amount of Pt nanoparticles. The Co@NC decorated with 1 wt% Pt exhibits the best ability for CO2 reduction to CH4 and a CH4 production rate of 14.4 mu mol.g(-1). h(-1) is achieved. It is worth noting that the system is carried out under low-concentration CO2 (400 ppm) circumstance without any sacrificial agent, which could be meaningful to the design of catalysts for atmospheric CO2 reduction. (C) 2018 Published by Elsevier Ltd on behalf of The editorial office of Journal of Materials Science & Technology. |
学科主题 | Materials Science, Multidisciplinary ; Metallurgy & Metallurgical Engineering |
WOS记录号 | WOS:000443274500015 |
出版者 | JOURNAL MATER SCI TECHNOL |
资助机构 | This work was financially supported by the National Natural Science Foundation of China (Nos. 51772312 and 51472260), the Environmental Functional Materials Innovation Team of Ministry of Education (IRT_16R49), and the International Joint Laboratory on Resource Chemistry (IJLRC). ; This work was financially supported by the National Natural Science Foundation of China (Nos. 51772312 and 51472260), the Environmental Functional Materials Innovation Team of Ministry of Education (IRT_16R49), and the International Joint Laboratory on Resource Chemistry (IJLRC). |
源URL | [http://ir.sic.ac.cn/handle/331005/24625] ![]() |
专题 | 中国科学院上海硅酸盐研究所 |
作者单位 | 1.Shanghai Normal Univ, Shanghai Key Lab Rare Earth Funct Mat, Key Lab Resource Chem, Minist Educ, Shanghai 200234, Peoples R China 2.Shanghai Normal Univ, Shanghai Municipal Educ Comm, Key Lab Mol Imaging Probes & Sensors, Shanghai 200234, Peoples R China 3.Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Super Fine, Shanghai 200050, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Qianqian,Wang, Wenzhong,Zhang, Ling,et al. Catalytic reduction of low-concentration CO2 with water by Pt/Co@NC[J]. JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,2018,34(12):2337, 2341. |
APA | Wang, Qianqian,Wang, Wenzhong,Zhang, Ling,Su, Yang,Wang, Kefu,&Wu, Huixia.(2018).Catalytic reduction of low-concentration CO2 with water by Pt/Co@NC.JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,34(12),2337. |
MLA | Wang, Qianqian,et al."Catalytic reduction of low-concentration CO2 with water by Pt/Co@NC".JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY 34.12(2018):2337. |
入库方式: OAI收割
来源:上海硅酸盐研究所
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