Temperature stable microwave dielectric ceramics in Li2ZnTi3O8-based composite for LTCC applications
文献类型：期刊论文
| 作者 | Ren, Haishen1; Peng, Haiyi2; Xie, Tianyi; Hao, Liang; Dang, Mingzhao2; Meng, Xie1; Jiang, Shaohu; Zhang, Yi; Lin, Huixing; Luo, Lan |
| 刊名 | JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
 |
| 出版日期 | 2018 |
| 卷号 | 29期号:15页码:12978 |
| ISSN号 | 0957-4522 |
| DOI | 10.1007/s10854-018-9418-0 |
| 英文摘要 | A temperature stable low temperature co-fired ceramic (LTCC) was fabricated by the powder mixture of Li2ZnTi3O8 ceramic, TiO2 tau(f)-tailoring dopant and B2O3-La2O3-MgO-TiO2 (BLMT) glass sintering aid, and the sintering behavior, activation energy, phase composition, microstructure and microwave dielectric properties of the composite were investigated in the composition range (wt%) of 5 BLMT-(95-x) Li2ZnTi3O8-X TiO2 (x = 0, 1, 2, 3, 4 and 5). The sintering behavior results showed that all composites could be well sintered at 910 A degrees C for 2 h through liquid-phase sintering. The activation energy of Li2ZnTi3O8 ceramic was calculated to be 520.9 +/- 40.46 kJ/mol, while 5BLMT-93Li(2)ZnTi(3)O(8)-2TiO(2) (in wt%) composite was reduced to 330.98 +/- 47.34 kJ/mol. The XRD results showed that Li2ZnTi3O8 and TiO2 phase stably existed in all sample and a new phase LaBO3 was crystallized from BLMT glass during sintering process. As x increases, the rutile TiO2 phase increased in composite, which could adjust the temperature coefficient of resonant frequency (tau(f)) to near-zero owing to the opposite tau(f) value to other phases. And simultaneously dielectric constant (epsilon(r)) demonstrated gradually increase, whereas the quality factor (Q x f) decreased gradually. The composite with x = 2 had an optimal microwave dielectric properties with epsilon(r) = 25.3, Q x f = 32,800 GHz, and tau(f) = - 0.54 ppm/A degrees C. The corresponding fitting equations of epsilon(r), Q x f and tau(f) on the x value were obtained by the Origin software, indicating that the dielectric properties of the composite could be precisely controlled by varying the content of TiO2. In addition, the good chemical compatibility of this material with Ag electrode made it as a potential candidate for LTCC technology. |
| 学科主题 | Engineering, Electrical & Electronic ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter |
| 出版者 | SPRINGER |
| WOS记录号 | WOS:000438679000051 |
| 源URL | [http://ir.sic.ac.cn/handle/331005/24766]  |
| 专题 | 中国科学院上海硅酸盐研究所 |
| 作者单位 | 1.Chinese Acad Sci, Shanghai Inst Ceram, Key Lab Inorgan Funct Mat & Device, Shanghai 200050, Peoples R China 2.Chinese Acad Sci, CAS Key Lab Mat Energy Convers, Shanghai 200050, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Ren, Haishen,Peng, Haiyi,Xie, Tianyi,et al. Temperature stable microwave dielectric ceramics in Li2ZnTi3O8-based composite for LTCC applications[J]. JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS,2018,29(15):12978, 12985. |
| APA | Ren, Haishen.,Peng, Haiyi.,Xie, Tianyi.,Hao, Liang.,Dang, Mingzhao.,...&Luo, Lan.(2018).Temperature stable microwave dielectric ceramics in Li2ZnTi3O8-based composite for LTCC applications.JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS,29(15),12978. |
| MLA | Ren, Haishen,et al."Temperature stable microwave dielectric ceramics in Li2ZnTi3O8-based composite for LTCC applications".JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS 29.15(2018):12978. |
入库方式： OAI收割
来源：上海硅酸盐研究所
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