Anion-Containing Noble-Metal-Free Bifunctional Electrocatalysts for Overall Water Splitting
文献类型：期刊论文
| 作者 | Xiong, Bingyan; Chen, Lisong; Shi, Jianlin1 |
| 刊名 | ACS CATALYSIS
 |
| 出版日期 | 2018 |
| 卷号 | 8期号:4页码:3688 |
| 关键词 | anion-containing noble-metal-free bifunctional electrocatalyst overall water-splitting energy conversion |
| ISSN号 | 2155-5435 |
| DOI | 10.1021/acscatal.7b04286 |
| 英文摘要 | With ever-increasing severe environment pollutions and energy demand, it is becoming greatly important to develop sustainable energy resources as alternatives to traditional fossil fuels. As one of the ultimate clean energy sources, hydrogen (H-2) energy produced by water splitting using electricity from solar radiation, wind, tide, and nuclear fusion, among other sources, has attracted more and more public attention since the late 18th century. Although noble-metal based electrocatalysts perform well, they suffer severely from the high cost and rarity from the viewpoint of practical applications. Recently, various kinds of non-noble-metal electrocatalysts based on low cost and earth-abundant transition metals have been developed for both hydrogen evolution reaction (HER) and oxygen (O-2) evolution reaction (OER). Among them, non-noble-metal bifunctional electrocatalysts (NHOBEs), showing high performances in both HER and OER, are therefore of great significance and importance in future applications. With NHOBEs, one will be able to significantly simplify the fabrication procedures of electrolyzers, and more importantly, elevate the efficiency of "all in one" electrocatalytic water-splitting systems, which will greatly favor their industrial applications by demanding substantially lowered the production costs. While the laws of NHOBEs from the same main group anionic elements such as oxygen, nitrogen, carbon, and boron families have not been well-reported so far. Herein, the recent significant progresses of NHOBEs classified by different main group anionic elements are summarized, and emphases are placed to the designs, syntheses, electrocatalytic performances in water-splitting, and future possible applications of NHOBEs. Moreover, the prospects of a number of vigorously investigated NHOBE catalysts and the possible trends of future developments are also evaluated. In addition, current challenges facing research with respect to electrocatalysts for water-splitting are discussed. |
| 学科主题 | Chemistry, Physical |
| WOS记录号 | WOS:000430154100112 |
| 出版者 | AMER CHEMICAL SOC |
| 资助机构 | This work was financially supported by National Natural Science Foundation of China (51702099), Shanghai Sailing Program (17YF1403800), China Postdoctoral Science Foundation funded project (2017M611500), Opening Project of State Key Laboratory of High Performance Ceramics and Superfine Microstructure (SKL201702SIC). ; This work was financially supported by National Natural Science Foundation of China (51702099), Shanghai Sailing Program (17YF1403800), China Postdoctoral Science Foundation funded project (2017M611500), Opening Project of State Key Laboratory of High Performance Ceramics and Superfine Microstructure (SKL201702SIC). |
| 源URL | [http://ir.sic.ac.cn/handle/331005/25026]  |
| 专题 | 中国科学院上海硅酸盐研究所 |
| 作者单位 | 1.East China Normal Univ, Sch Chem & Mol Engn, Shanghai Key Lab Green Chem & Chem Proc, Shanghai 200062, Peoples R China 2.Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China |
| 推荐引用方式 GB/T 7714 | Xiong, Bingyan,Chen, Lisong,Shi, Jianlin. Anion-Containing Noble-Metal-Free Bifunctional Electrocatalysts for Overall Water Splitting[J]. ACS CATALYSIS,2018,8(4):3688, 3707. |
| APA | Xiong, Bingyan,Chen, Lisong,&Shi, Jianlin.(2018).Anion-Containing Noble-Metal-Free Bifunctional Electrocatalysts for Overall Water Splitting.ACS CATALYSIS,8(4),3688. |
| MLA | Xiong, Bingyan,et al."Anion-Containing Noble-Metal-Free Bifunctional Electrocatalysts for Overall Water Splitting".ACS CATALYSIS 8.4(2018):3688. |
入库方式： OAI收割
来源：上海硅酸盐研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。