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Depth dependant element analysis of PbMg1/3Nb2/3O3 using muonic x-rays

文献类型:期刊论文

作者Brown, K. L.; Stockdale, C. P. J.; Luo, H.; Zhao, X.; Li, J-F; Viehland, D.; Xu, G.; Gehring, P. M.; Ishida, K.; Hillier, A. D.
刊名JOURNAL OF PHYSICS-CONDENSED MATTER
出版日期2018
卷号30期号:12
ISSN号0953-8984
关键词ferroelectricity domains composition muonic x-rays structural order parameter
DOI10.1088/1361-648X/aaade3
英文摘要The relaxor PbMg1/3Nb2/3O3 (PMN) has received attention due to its potential applications as a piezoelectric when doped with PbTiO3 (PT). Previous results have found that there are two phases existing in the system, one linked to the near-surface regions of the sample, the other in the bulk. However, the exact origin of these two phases is unclear. In this paper, depth dependant analysis results from negative muon implantation experiments are presented. It is shown that the Pb content is constant throughout all depths probed in the sample, but the Mg and Nb content changes in the near-surface region below 100 mu m. At an implantation depth of 60 mu m, it is found that there is a 25% increase in Mg content, with a simultaneous 5% decrease in Nb content in order to maintain charge neutrality. These results show that the previously observed skin effects in PMN are due to a change in concentration and unit cell.
学科主题Physics, Condensed Matter
出版者IOP PUBLISHING LTD
WOS记录号WOS:000426476800001
资助机构Support is gratefully acknowledged from the EPSRC, the STFC, the Royal Society, and the Carnegie Trust for the Universities of Scotland. ; Support is gratefully acknowledged from the EPSRC, the STFC, the Royal Society, and the Carnegie Trust for the Universities of Scotland.
源URL[http://ir.sic.ac.cn/handle/331005/25080]  
专题中国科学院上海硅酸盐研究所
作者单位1.[Brown, K. L.
2.Stockdale, C. P. J.
3.Stock, C.] Univ Edinburgh, Sch Phys & Astron, Edinburgh EH9 3JZ, Midlothian, Scotland
4.[Luo, H.] Chinese Acad Sci, Shanghai Inst Ceram, Shanghai 201800, Peoples R China
5.[Zhao, X.] Shanghai Normal Univ, Shanghai 200234, Peoples R China
6.[Li, J-F
7.Viehland, D.] Virginia Tech, Dept Mat Sci & Engn, Blacksburg, VA 24061 USA
8.[Xu, G.
9.Gehring, P. M.] NIST, Gaithersburg, MD USA
10.[Ishida, K.] RIKEN, Nishina Ctr, Wako, Saitama, Japan
推荐引用方式
GB/T 7714
Brown, K. L.,Stockdale, C. P. J.,Luo, H.,et al. Depth dependant element analysis of PbMg1/3Nb2/3O3 using muonic x-rays[J]. JOURNAL OF PHYSICS-CONDENSED MATTER,2018,30(12).
APA Brown, K. L..,Stockdale, C. P. J..,Luo, H..,Zhao, X..,Li, J-F.,...&Stock, C..(2018).Depth dependant element analysis of PbMg1/3Nb2/3O3 using muonic x-rays.JOURNAL OF PHYSICS-CONDENSED MATTER,30(12).
MLA Brown, K. L.,et al."Depth dependant element analysis of PbMg1/3Nb2/3O3 using muonic x-rays".JOURNAL OF PHYSICS-CONDENSED MATTER 30.12(2018).

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来源:上海硅酸盐研究所

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