中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Insight into excitation-related luminescence properties of carbon dots: synergistic effect from photoluminescence centers in the carbon core and on the surface

文献类型:期刊论文

作者Li, Bo1,2; Guo, Yali1; Iqbal, Anam1; Dong, Yaping2; Li, Wu2; Liu, Weisheng1; Qin, Wenwu1; Wang, Yabin2,3
刊名RSC ADVANCES
出版日期2016
卷号6期号:109页码:107263-107269
文献子类Article
英文摘要Excitation-dependent luminescence (EDE) or excitation-independent luminescence (EIE) property of carbon dots (CDs) has attracted considerable attention. For the first time, we found that nitrogen doped CDs possess adjustable EDE and EIE properties by changing the corresponding environmental pH values for photoluminescence (PL) properties. Structural characterizations and property tests demonstrate that the unique photoluminescence properties of CDs can be attributed to the synergistic effect from the PL centers in the carbon core and on the surface. Doping nitrogen into the carbon core improves the emission efficiency of PL centers; these enhanced PL sites can even dominate fluorescence emission. Passivated surfaces of CDs modified with amino groups not only further boost the emission efficiency, but also make energy levels of PL centers more uniform. In addition, the mechanism of synergistic effect is investigated, which opens up the possibility of designing CDs with desirable PL characteristics. Such nitrogen-doped CDs with adjustable excitation-related luminescence properties have potential applications in detecting acidity or alkalinity of a certain physiological environment by intuitively observing the change in the wavelength.
WOS关键词GRAPHENE QUANTUM DOTS ; FULL-COLOR EMISSION ; ONE-STEP SYNTHESIS ; PHOTOCATALYTIC ACTIVITY ; INDEPENDENT EMISSION ; BLUE LUMINESCENCE ; DEEP-ULTRAVIOLET ; NITROGEN ; FLUORESCENCE ; LIGHT
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000389342400015
源URL[http://ir.isl.ac.cn/handle/363002/6177]  
专题青海盐湖研究所_青海盐湖研究所知识仓储
青海盐湖研究所_盐湖资源综合利用工程技术中心
作者单位1.Lanzhou Univ, Key Lab Nonferrous Met Chem & Resources Utilizat, Lanzhou 730000, Peoples R China
2.Chinese Acad Sci, Qinghai Inst Salt Lakes, Xining 810008, Qinghai, Peoples R China
3.Harbin Inst Technol, Sch Chem & Chem Engn, Harbin 150001, Peoples R China
推荐引用方式
GB/T 7714
Li, Bo,Guo, Yali,Iqbal, Anam,et al. Insight into excitation-related luminescence properties of carbon dots: synergistic effect from photoluminescence centers in the carbon core and on the surface[J]. RSC ADVANCES,2016,6(109):107263-107269.
APA Li, Bo.,Guo, Yali.,Iqbal, Anam.,Dong, Yaping.,Li, Wu.,...&Wang, Yabin.(2016).Insight into excitation-related luminescence properties of carbon dots: synergistic effect from photoluminescence centers in the carbon core and on the surface.RSC ADVANCES,6(109),107263-107269.
MLA Li, Bo,et al."Insight into excitation-related luminescence properties of carbon dots: synergistic effect from photoluminescence centers in the carbon core and on the surface".RSC ADVANCES 6.109(2016):107263-107269.

入库方式: OAI收割

来源:青海盐湖研究所

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