中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Reactivity of sewage sludge, RDF, and straw chars towards NO

文献类型:期刊论文

作者Ulusoy, Burak1,2; Wu, Hao1; Lin, Weigang1,3; Karlstrom, Oskar4; Li, Songgeng3,5; Song, Wenli3,5; Glarborg, Peter1; Dam-Johansen, Kim1
刊名FUEL
出版日期2019-01-15
卷号236页码:297-305
关键词NO reduction Char reactivity Waste combustion Sewage sludge Refuse derived fuel
ISSN号0016-2361
DOI10.1016/j.fuel.2018.08.164
英文摘要The reaction of NO with chars of sewage sludge, refuse derived fuel (RDF), and straw was investigated in a fixed bed reactor at temperatures from 800 to 900 degrees C and NO inlet concentrations from 400 to 1500 ppmv. The effect of ash forming elements in the chars was examined by comparing the reactivity of raw and demineralized chars. Compared to straw char, the reaction rates of sewage sludge and RDF char, at 800 degrees C and 400 ppmv inlet NO, was an order of magnitude and a factor of six higher, respectively. The very high reactivity of the two waste chars was attributed to the catalytic effect of their large content of calcium and iron. A simple first order globalized rate expression was employed to describe the reactivity of waste chars toward NO, which predicted reasonably well the the conversion of char nitrogen to NO during char combustion at 800 degrees C in 10% O-2. A comparison with literature data revealed a higher reactivity of the waste chars towards NO compared to that of coal and biomass chars. The results in this work provide a simple and validated rate expression to simulate waste char-NO reaction in boilers, and moreover facilitate a potential utilization of waste chars as primary or secondary measures for NO reduction.
WOS关键词FLUIDIZED-BED COMBUSTION ; HIGH-TEMPERATURE ; BIOMASS CHAR ; COAL CHARS ; NITROGEN CONVERSION ; FIXED-BED ; REDUCTION ; OXIDATION ; CARBON ; AIR
资助项目Sino-Danish Centre for Education and Research ; Academy of Finland[289666] ; Technical University of Denmark
WOS研究方向Energy & Fuels ; Engineering
语种英语
WOS记录号WOS:000447799400028
出版者ELSEVIER SCI LTD
资助机构Sino-Danish Centre for Education and Research ; Academy of Finland ; Technical University of Denmark
源URL[http://ir.ipe.ac.cn/handle/122111/26178]  
专题中国科学院过程工程研究所
通讯作者Wu, Hao
作者单位1.Tech Univ Denmark, Dept Chem & Biochem Engn, Soltofts Plads 229, DK-2800 Lyngby, Denmark
2.Sino Danish Ctr Educ & Res, Beijing, Peoples R China
3.Univ Chinese Acad Sci, Sino Danish Coll, Beijing 100049, Peoples R China
4.Abo Akad Univ, Johan Gadolin Proc Chem, Turku, Finland
5.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714
Ulusoy, Burak,Wu, Hao,Lin, Weigang,et al. Reactivity of sewage sludge, RDF, and straw chars towards NO[J]. FUEL,2019,236:297-305.
APA Ulusoy, Burak.,Wu, Hao.,Lin, Weigang.,Karlstrom, Oskar.,Li, Songgeng.,...&Dam-Johansen, Kim.(2019).Reactivity of sewage sludge, RDF, and straw chars towards NO.FUEL,236,297-305.
MLA Ulusoy, Burak,et al."Reactivity of sewage sludge, RDF, and straw chars towards NO".FUEL 236(2019):297-305.

入库方式: OAI收割

来源:过程工程研究所

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