Core-shell LaPO4/g-C3N4nanowires for highly active and selective CO2reduction
文献类型:期刊论文
作者 | Li, Mengli2; Zhang, Lingxia1; Fan, Xiangqian1; Wu, Meiying1; Wang, Min1; Cheng, Ruolin1; Zhang, Linlin1; Yao, Heliang1; Shi, Jianlin1,3 |
刊名 | Applied Catalysis B: Environmental
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出版日期 | 2017 |
卷号 | 201页码:629-635 |
ISSN号 | 09263373 |
DOI | 10.1016/j.apcatb.2016.09.004 |
英文摘要 | We have synthesized a series of LaPO4/g-C3N4core-shell nanowires via an in-situ hydrothermal growth of LaPO4nanorods in tubular g-C3N4and investigated their photocatalytic activity in CO2reduction. It was found that in the synthesized core-shell structure, the outer g-C3N4nano-shells coated on the LaPO4nanorod cores resulted in the enhanced light absorption and charge carrier separation/transfer ability, thus improved the room temperature photocatalytic performance of the nanocomposites in CO2photocatalytic reduction compared with the g-C3N4and LaPO4individuals. A maximum CO yield of 0.433 μmol has been obtained from CO2reduction within 1 h irradiation on 30 mg nanocomposite photocatalyst under the absence of any noble metal. Finally, a possible mechanism, which is featured with LaPO4activation due to significantly promoted separation/transfer of photo-generated charge carriers, was proposed. The encouraging performance in CO2photoreduction demonstrates that this novel nanocomposite will be a prospective material in environmental protection and energy conversion. © 2016 |
源URL | [http://ir.sic.ac.cn/handle/331005/25805] ![]() |
专题 | 中国科学院上海硅酸盐研究所 |
作者单位 | 1.State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, 1295 Ding-Xi Road, Shanghai; 200050, China; 2.School of Biology and Chemical Engineering, Jiaxing University, Jiaxing; Zhejiang; 314001, China; 3.Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), China |
推荐引用方式 GB/T 7714 | Li, Mengli,Zhang, Lingxia,Fan, Xiangqian,et al. Core-shell LaPO4/g-C3N4nanowires for highly active and selective CO2reduction[J]. Applied Catalysis B: Environmental,2017,201:629-635. |
APA | Li, Mengli.,Zhang, Lingxia.,Fan, Xiangqian.,Wu, Meiying.,Wang, Min.,...&Shi, Jianlin.(2017).Core-shell LaPO4/g-C3N4nanowires for highly active and selective CO2reduction.Applied Catalysis B: Environmental,201,629-635. |
MLA | Li, Mengli,et al."Core-shell LaPO4/g-C3N4nanowires for highly active and selective CO2reduction".Applied Catalysis B: Environmental 201(2017):629-635. |
入库方式: OAI收割
来源:上海硅酸盐研究所
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