Numerical investigation of Lower Tuscaloosa Sandstone and Selma Chalk caprock under geological CO2 sequestration conditions: mineral precipitation and permeability evolution
文献类型：期刊论文
| 作者 | Zhang, Liwei1,2; Soong, Yee3; Dilmore, Robert M.3 |
| 刊名 | GREENHOUSE GASES-SCIENCE AND TECHNOLOGY
 |
| 出版日期 | 2017 |
| 卷号 | 7期号:6页码:988-1007 |
| 关键词 | geologic carbon sequestration amorphous silica kaolinite porosity permeability reactive transport modeling brine Tuscaloosa Formation |
| ISSN号 | 2152-3878 |
| DOI | 10.1002/ghg.1703 |
| 英文摘要 | A numerical model was developed using CrunchFlow to simulate reactive transport and porosity and permeability changes of sandstone and carbonate rock samples taken from the Lower Tuscaloosa Formation and the Selma Chalk Formation, Jackson County, MS, USA. The model predicted a permeability decrease from 2190 mD to 2038 mD for the Lower Tuscaloosa Sandstone sample in a static batch reactor after 180 days of exposure to CO2-saturated brine, which is consistent with measured permeability results. The model predicted a negligible permeability change from 2.00 mD to 2.08 mD for the Selma Chalk carbonate sample after 180 days of exposure to CO2-saturated brine. Based on model prediction, key mineral dissolution and precipitation reactions in the Lower Tuscaloosa Sandstone sample include dissolution of quartz, chlorite, and feldspar, as well as precipitation of amorphous silica and kaolinite. For the Selma Chalk carbonate sample, key predicted reactions include dissolution of calcite, quartz and chlorite, and precipitation of kaolinite and amorphous silica. Initial porosity, initial feldspar content and the exponent n value (related to pore structure and tortuosity) used in permeability calculations were three important factors affecting permeability evolution of sandstone samples under CO2 sequestration conditions. The small permeability change predicted for both the Lower Tuscaloosa Sandstone and the Selma Chalk caprock after exposure to CO2-saturated brine suggests that poro-permeability changes during CO2 injection into the Lower Tuscaloosa Formation are not likely to significantly affect reservoir and seal quality. (c) 2017 Society of Chemical Industry and John Wiley & Sons, Ltd. |
| WOS研究方向 | Energy & Fuels ; Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:000417761600004 |
| 出版者 | WILEY PERIODICALS, INC |
| 源URL | [http://119.78.100.198/handle/2S6PX9GI/4173]  |
| 专题 | 岩土力学所知识全产出_期刊论文 国家重点实验室知识产出_期刊论文 |
| 作者单位 | 1.Chinese Acad Sci, State Key Lab Geomech & Geotech Engn, IRSM ; 2.NETL, ORISE, Pittsburgh, PA USA; 3.US DOE, NETL |
| 推荐引用方式 GB/T 7714 | Zhang, Liwei,Soong, Yee,Dilmore, Robert M.. Numerical investigation of Lower Tuscaloosa Sandstone and Selma Chalk caprock under geological CO2 sequestration conditions: mineral precipitation and permeability evolution[J]. GREENHOUSE GASES-SCIENCE AND TECHNOLOGY,2017,7(6):988-1007. |
| APA | Zhang, Liwei,Soong, Yee,&Dilmore, Robert M..(2017).Numerical investigation of Lower Tuscaloosa Sandstone and Selma Chalk caprock under geological CO2 sequestration conditions: mineral precipitation and permeability evolution.GREENHOUSE GASES-SCIENCE AND TECHNOLOGY,7(6),988-1007. |
| MLA | Zhang, Liwei,et al."Numerical investigation of Lower Tuscaloosa Sandstone and Selma Chalk caprock under geological CO2 sequestration conditions: mineral precipitation and permeability evolution".GREENHOUSE GASES-SCIENCE AND TECHNOLOGY 7.6(2017):988-1007. |
入库方式： OAI收割
来源：武汉岩土力学研究所
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