An integrated air-POM syngas/dimethyl ether process from natural gas
文献类型：期刊论文
| 作者 | Jia, ML; Li, WZ; Xu, HY; Hou, SF; Ge, QJ |
| 刊名 | applied catalysis a-general
 |
| 出版日期 | 2002-07-10 |
| 卷号 | 233期号:1-2页码:7-12 |
| 关键词 | syngas dimethyl ether catalytic partial oxidation of methane |
| 英文摘要 | a cu-zn-al methanol catalyst combined with hzsm-5 was used for dimethyl ether (dme) synthesis from a syngas containing nitrogen, which was produced by air-partial oxidation of methane (air-pom). air-pom occurred at 850 degreesc, 0.8 mpa, ch4/air/h2o/co2 ratio of 1/2.4/0.8/0.4 over a ni-based catalyst modified by magnesia and lanthanum oxide with 96% ch4 conversion and constantly gave syngas with a h-2/co ratio of 2/1 during a period of 450 h. the obtained n-2-containing syngas was used directly for dme synthesis. about 90% co per-pass conversion, 78% dme selectivity and 70% dme yield could be achieved during 450 h stability testing under the pressure of 5.0 mpa. the temperature of 240 degreesc and the space velocity of 1000 h(-1). (c) 2002 elsevier science b. v. all rights reserved. |
| WOS标题词 | science & technology ; physical sciences ; life sciences & biomedicine |
| 类目[WOS] | chemistry, physical ; environmental sciences |
| 研究领域[WOS] | chemistry ; environmental sciences & ecology |
| 关键词[WOS] | dimethyl ether ; syngas ; catalysts ; methanol ; oxidation |
| 收录类别 | SCI |
| 原文出处 | true |
| 语种 | 英语 |
| WOS记录号 | WOS:000176787400002 |
| 公开日期 | 2010-11-30 |
| 源URL | [http://159.226.238.44/handle/321008/85755]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China |
| 推荐引用方式 GB/T 7714 | Jia, ML,Li, WZ,Xu, HY,et al. An integrated air-POM syngas/dimethyl ether process from natural gas[J]. applied catalysis a-general,2002,233(1-2):7-12. |
| APA | Jia, ML,Li, WZ,Xu, HY,Hou, SF,&Ge, QJ.(2002).An integrated air-POM syngas/dimethyl ether process from natural gas.applied catalysis a-general,233(1-2),7-12. |
| MLA | Jia, ML,et al."An integrated air-POM syngas/dimethyl ether process from natural gas".applied catalysis a-general 233.1-2(2002):7-12. |
入库方式： OAI收割
来源：大连化学物理研究所
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