Can i-129 track cs-135, u-236, pu-239, and pu-240 apart from i-131 in soil samples from fukushima prefecture, japan?
文献类型:期刊论文
作者 | Yang, Guosheng1,2,3; Tazoe, Hirofumi1; Yamada, Masatoshi1 |
刊名 | Scientific reports
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出版日期 | 2017-11-13 |
卷号 | 7页码:7 |
ISSN号 | 2045-2322 |
DOI | 10.1038/s41598-017-15714-w |
通讯作者 | Yamada, masatoshi(myamada@hirosaki-u.ac.jp) |
英文摘要 | In the present study, i-129 activities and i-129/i-127 atom ratios were measured in 60 soil samples contaminated by the fukushima daiichi nuclear power plant (fdnpp) accident. the i-127 concentrations, i-129 activities, and i-129/i-127 atom ratios in dry-weight were observed to be 0.121-23.6 mg kg(-1), 0.962-275 mbq kg(-1), and (0.215-79.3) x 10(-7), respectively. the maximum values of both i-129 activities and i-129/i-127 atom ratios in japanese soil increased about three orders of magnitude due to this accident. the equation logy = 0.877logx + 0.173 (pearson's r = 0.936; x, i-129 concentration; y, i-131 concentration; decay-corrected to march 11, 2011) instead of a simple constant may be a better way to express the relationship between i-129 and i-131 in japanese soil affected by both global fallout and fdnpp accident fallout. in addition, a moderate correlation was observed between i-129 and cs-135 (logy = 0.624logx + 1.01, pearson's r = 0.627; x, i-129 activity; y, cs-135 activity). however, i-129 presented larger fractionations with less volatile radionuclides, such as u-236, pu-239, and pu-240. these findings indicated cs-135 could be roughly estimated from i-129 or i-131; this is advantageous as fewer cs-135 data are available and cs-135/cs-137 is being considered a promising tracer during radiocesium source identification. |
WOS关键词 | NUCLEAR-POWER-PLANT ; ACCELERATOR MASS-SPECTROMETRY ; ENVIRONMENTAL-SAMPLES ; ATMOSPHERIC FALLOUT ; ISOTOPIC RATIO ; PU ISOTOPES ; ACCIDENT ; RADIONUCLIDES ; SYSTEM |
WOS研究方向 | Science & Technology - Other Topics |
WOS类目 | Multidisciplinary Sciences |
语种 | 英语 |
WOS记录号 | WOS:000415022900005 |
出版者 | NATURE PUBLISHING GROUP |
URI标识 | http://www.irgrid.ac.cn/handle/1471x/2176896 |
专题 | 高能物理研究所 |
通讯作者 | Yamada, Masatoshi |
作者单位 | 1.Hirosaki Univ, Inst Radiat Emergency Med, Dept Radiat Chem, 66-1 Hon Cho, Hirosaki, Aomori 0368564, Japan 2.Chinese Acad Sci, Inst High Energy Phys, Div Nucl Technol & Applicat, Beijing, Peoples R China 3.Beijing Engn Res Ctr Radiog Tech & Equipment, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Yang, Guosheng,Tazoe, Hirofumi,Yamada, Masatoshi. Can i-129 track cs-135, u-236, pu-239, and pu-240 apart from i-131 in soil samples from fukushima prefecture, japan?[J]. Scientific reports,2017,7:7. |
APA | Yang, Guosheng,Tazoe, Hirofumi,&Yamada, Masatoshi.(2017).Can i-129 track cs-135, u-236, pu-239, and pu-240 apart from i-131 in soil samples from fukushima prefecture, japan?.Scientific reports,7,7. |
MLA | Yang, Guosheng,et al."Can i-129 track cs-135, u-236, pu-239, and pu-240 apart from i-131 in soil samples from fukushima prefecture, japan?".Scientific reports 7(2017):7. |
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来源:高能物理研究所
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