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Can i-129 track cs-135, u-236, pu-239, and pu-240 apart from i-131 in soil samples from fukushima prefecture, japan?

文献类型:期刊论文

作者Yang, Guosheng1,2,3; Tazoe, Hirofumi1; Yamada, Masatoshi1
刊名Scientific reports
出版日期2017-11-13
卷号7页码:7
ISSN号2045-2322
DOI10.1038/s41598-017-15714-w
通讯作者Yamada, masatoshi(myamada@hirosaki-u.ac.jp)
英文摘要In the present study, i-129 activities and i-129/i-127 atom ratios were measured in 60 soil samples contaminated by the fukushima daiichi nuclear power plant (fdnpp) accident. the i-127 concentrations, i-129 activities, and i-129/i-127 atom ratios in dry-weight were observed to be 0.121-23.6 mg kg(-1), 0.962-275 mbq kg(-1), and (0.215-79.3) x 10(-7), respectively. the maximum values of both i-129 activities and i-129/i-127 atom ratios in japanese soil increased about three orders of magnitude due to this accident. the equation logy = 0.877logx + 0.173 (pearson's r = 0.936; x, i-129 concentration; y, i-131 concentration; decay-corrected to march 11, 2011) instead of a simple constant may be a better way to express the relationship between i-129 and i-131 in japanese soil affected by both global fallout and fdnpp accident fallout. in addition, a moderate correlation was observed between i-129 and cs-135 (logy = 0.624logx + 1.01, pearson's r = 0.627; x, i-129 activity; y, cs-135 activity). however, i-129 presented larger fractionations with less volatile radionuclides, such as u-236, pu-239, and pu-240. these findings indicated cs-135 could be roughly estimated from i-129 or i-131; this is advantageous as fewer cs-135 data are available and cs-135/cs-137 is being considered a promising tracer during radiocesium source identification.
WOS关键词NUCLEAR-POWER-PLANT ; ACCELERATOR MASS-SPECTROMETRY ; ENVIRONMENTAL-SAMPLES ; ATMOSPHERIC FALLOUT ; ISOTOPIC RATIO ; PU ISOTOPES ; ACCIDENT ; RADIONUCLIDES ; SYSTEM
WOS研究方向Science & Technology - Other Topics
WOS类目Multidisciplinary Sciences
语种英语
WOS记录号WOS:000415022900005
出版者NATURE PUBLISHING GROUP
URI标识http://www.irgrid.ac.cn/handle/1471x/2176896
专题高能物理研究所
通讯作者Yamada, Masatoshi
作者单位1.Hirosaki Univ, Inst Radiat Emergency Med, Dept Radiat Chem, 66-1 Hon Cho, Hirosaki, Aomori 0368564, Japan
2.Chinese Acad Sci, Inst High Energy Phys, Div Nucl Technol & Applicat, Beijing, Peoples R China
3.Beijing Engn Res Ctr Radiog Tech & Equipment, Beijing 100049, Peoples R China
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Yang, Guosheng,Tazoe, Hirofumi,Yamada, Masatoshi. Can i-129 track cs-135, u-236, pu-239, and pu-240 apart from i-131 in soil samples from fukushima prefecture, japan?[J]. Scientific reports,2017,7:7.
APA Yang, Guosheng,Tazoe, Hirofumi,&Yamada, Masatoshi.(2017).Can i-129 track cs-135, u-236, pu-239, and pu-240 apart from i-131 in soil samples from fukushima prefecture, japan?.Scientific reports,7,7.
MLA Yang, Guosheng,et al."Can i-129 track cs-135, u-236, pu-239, and pu-240 apart from i-131 in soil samples from fukushima prefecture, japan?".Scientific reports 7(2017):7.

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来源:高能物理研究所

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