Directed biofabrication of nanoparticles through regulating extracellular electron transfer
文献类型：期刊论文
| 作者 | Tian, Li-Jiao1; Li, Wen-Wei1; Zhu, Ting-Ting1; Chen, Jie-Jie1; Wang, Wei-Kang1; An, Peng-Fei3; Zhang, Long3; Dong, Jun-Cai3; Guan, Yong2; Liu, Dong-Feng1 |
| 刊名 | Journal of the american chemical society
 |
| 出版日期 | 2017-09-06 |
| 卷号 | 139期号:35页码:12149-12152 |
| ISSN号 | 0002-7863 |
| DOI | 10.1021/jacs.7b07460 |
| 通讯作者 | Li, wen-wei(wwli@ustc.edu.cn) ; Yu, han-qing(hqyu@ustc.edu.cn) |
| 英文摘要 | Biofabrication of nanomaterials is currently constrained by a low production efficiency and poor controllability on product quality compared to chemical synthetic routes. in this work, we show an attractive new biosynthesis system to break these limitations. a directed production of selenium-containing nanoparticles in shewanella oneidensis mr-1 cells, with fine-tuned composition and subcellular synthetic location, was achieved by modifying the extracellular electron transfer chain. by taking advantage of its untapped intracellular detoxification and synthetic power, we obtained high-purity, uniform sized cadmium selenide nanoparticles in the cytoplasm, with the production rates and fluorescent intensities far exceeding the state-of-the-art biosystems. these findings may fundamentally change our perception of nanomaterial biosynthesis process and lead to the development of fine controllable nanoparticles biosynthesis technologies. |
| WOS关键词 | QUANTUM DOTS ; MAGNETOTACTIC BACTERIA ; SHEWANELLA-ONEIDENSIS ; SELENIUM ; CELLS ; MECHANISMS ; DIVERSE ; MERCURY |
| WOS研究方向 | Chemistry |
| WOS类目 | Chemistry, Multidisciplinary |
| 语种 | 英语 |
| WOS记录号 | WOS:000410255600012 |
| 出版者 | AMER CHEMICAL SOC |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2177053 |
| 专题 | 高能物理研究所 |
| 通讯作者 | Li, Wen-Wei; Yu, Han-Qing |
| 作者单位 | 1.Univ Sci & Technol China, Dept Chem, CAS Key Lab Urban Pollutant Convers, Hefei 230026, Anhui, Peoples R China 2.Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230026, Anhui, Peoples R China 3.Chinese Acad Sci, Beijing Synchrotron Radiat Lab, Inst High Energy Phys, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Tian, Li-Jiao,Li, Wen-Wei,Zhu, Ting-Ting,et al. Directed biofabrication of nanoparticles through regulating extracellular electron transfer[J]. Journal of the american chemical society,2017,139(35):12149-12152. |
| APA | Tian, Li-Jiao.,Li, Wen-Wei.,Zhu, Ting-Ting.,Chen, Jie-Jie.,Wang, Wei-Kang.,...&Yu, Han-Qing.(2017).Directed biofabrication of nanoparticles through regulating extracellular electron transfer.Journal of the american chemical society,139(35),12149-12152. |
| MLA | Tian, Li-Jiao,et al."Directed biofabrication of nanoparticles through regulating extracellular electron transfer".Journal of the american chemical society 139.35(2017):12149-12152. |
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来源：高能物理研究所
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