Ce0.3zr0.7o1.88n0.12 solid solution as a stable photocatalyst for visible light driven water splitting
文献类型：期刊论文
| 作者 | Wang, Yu Lei1; Jin, Jia Min2,3; Li, Yu Hang1; Wang, Xue Lu1; Zhang, Bo4,5; Gong, Xiwen5; Wang, Hai Feng2,3; Chen, Ai Ping1; Zheng, Li Rong6; Hu, P.2,3,7 |
| 刊名 | Applied catalysis b-environmental
 |
| 出版日期 | 2018-05-01 |
| 卷号 | 224页码:733-739 |
| 关键词 | Photocatalysis Ce0.3zr0.7o1.88n0.12 Hydrogen evolution Z-scheme Stability |
| ISSN号 | 0926-3373 |
| DOI | 10.1016/j.apcatb.2017.11.012 |
| 通讯作者 | Yang, hua gui(hgyang@ecust.edu.cn) |
| 英文摘要 | The search of efficient and stable photocatalysts for the evolution of hydrogen from water using solar energy is of great importance for material science today. limited by the relatively inferior stability of oxynitrides, the availability of these visible-light-response materials in photocatalysis is still far below what is expected. here we report a novel oxynitride ce0.3zr0.7o1.88n0.12 as an efficient and stable h-2-evolving photocatalyst under visible light irradiation, which can further enable overall water splitting by coupling with an o-2-evolving photocatalyst via z-scheme. experimental and theoretical results together reveal that the origin of the excellent activity and stability of ce0.3zr0.7o1.88n0.12 photocatalyst can be attributed to the improved separation rate of photoexcited charge carriers by surface and sub-surface oxygen vacancies. the present study provides a strategy to engineer efficient and stable photocatalysts, and the oxynitride mentioned above could act as a promising candidate of h-2-evolving photocatalyst for designing a prominent z-scheme photocatalytic system. |
| WOS关键词 | DENSITY-FUNCTIONAL THEORY ; HYDROGEN-PRODUCTION ; OXYGEN DEFECTS ; CO OXIDATION ; PHOTOANODE ; EVOLUTION ; CATALYSTS ; SURFACE ; NANOPARTICLES ; IRRADIATION |
| WOS研究方向 | Chemistry ; Engineering |
| WOS类目 | Chemistry, Physical ; Engineering, Environmental ; Engineering, Chemical |
| 语种 | 英语 |
| WOS记录号 | WOS:000424960700076 |
| 出版者 | ELSEVIER SCIENCE BV |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2178033 |
| 专题 | 高能物理研究所 |
| 通讯作者 | Yang, Hua Gui |
| 作者单位 | 1.East China Univ Sci & Technol, Sch Mat Sci & Engn, Minist Educ, Key Lab Ultrafine Mat, 130 Meilong Rd, Shanghai 200237, Peoples R China 2.East China Univ Sci & Technol, Ctr Computat Chem, Key Lab Adv Mat, 130 Meilong Rd, Shanghai 200237, Peoples R China 3.East China Univ Sci & Technol, Res Inst Ind Catalysis, 130 Meilong Rd, Shanghai 200237, Peoples R China 4.Fudan Univ, Dept Macromol Sci, State Key Lab Mol Engn Polymers, Shanghai 200438, Peoples R China 5.Univ Toronto, Dept Elect & Comp Engn, 35 St George St, Toronto, ON M5S 1A4, Canada 6.Chinese Acad Sci, Inst High Energy Phys, Beijing Synchrotron Radiat Facil, Beijing 100049, Peoples R China 7.Queens Univ Belfast, Sch Chem & Chem Engn, Belfast BT9 5AG, Antrim, North Ireland |
| 推荐引用方式 GB/T 7714 | Wang, Yu Lei,Jin, Jia Min,Li, Yu Hang,et al. Ce0.3zr0.7o1.88n0.12 solid solution as a stable photocatalyst for visible light driven water splitting[J]. Applied catalysis b-environmental,2018,224:733-739. |
| APA | Wang, Yu Lei.,Jin, Jia Min.,Li, Yu Hang.,Wang, Xue Lu.,Zhang, Bo.,...&Yang, Hua Gui.(2018).Ce0.3zr0.7o1.88n0.12 solid solution as a stable photocatalyst for visible light driven water splitting.Applied catalysis b-environmental,224,733-739. |
| MLA | Wang, Yu Lei,et al."Ce0.3zr0.7o1.88n0.12 solid solution as a stable photocatalyst for visible light driven water splitting".Applied catalysis b-environmental 224(2018):733-739. |
入库方式： iSwitch采集
来源：高能物理研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。