Chlorine levels and species in fine and size resolved atmospheric particles by x-ray absorption near-edge structure spectroscopy analysis in beijing, china
文献类型：期刊论文
| 作者 | Ouyang, Jie1,2; Yang, Guo-Sheng3; Ma, Ling-Ling1; Luo, Min1; Zheng, Lei4; Huo, Qing5; Zhao, Yi-Dong4; Hu, Tian-Dou4; Cai, Zhen-Feng6; Xu, Dian-Dou1 |
| 刊名 | Chemosphere
 |
| 出版日期 | 2018-04-01 |
| 卷号 | 196页码:393-401 |
| 关键词 | Chlorine species Fine atmospheric particles X-ray absorption near edge structure (xanes) spectroscopy Size distribution Beijing |
| ISSN号 | 0045-6535 |
| DOI | 10.1016/j.chemosphere.2017.12.126 |
| 通讯作者 | Ma, ling-ling(malingling@ihep.ac.cn) ; Xu, dian-dou(xudd@ihep.ac.cn) |
| 英文摘要 | An understanding of the species of chlorine is crucial in the metropolis-beijing, which is suffering serious haze pollution with high frequency. particulate matters (pms) with five different sizes were collected in beijing from july 2009 to march 2016, and characterized non-destructively by x-ray absorption near edge structure spectroscopy. pm<0.2, pm0.2-0.5 and pm>2.5 contributed for the major pms mass in spring and summer, pm0.5-1.0 and pm1.0-25 contributed for the major pms mass in autumn and winter. the concentrations of the three chlorine species were in the order of inorganic chlorine (cl-inorg) > aliphatic chlorine (cl-ali) > aromatic chlorine (cl-aro), indicating that cl-inorg constituted the primary chlorine fraction and less toxic cl-ali constituted the primary total organic chlorine (cl-ali + cl-aro, abbreviated as cl-org) in the pms in beijing. in addition, these three chlorine species exhibited identical seasonal variation in pm2.5: winter > autumn> spring > summer. wet precipitation is an important factor to result in the lower mass concentrations of these three chlorine species in summer. the temporal variations of both size resolved pm mass concentrations and chlorine species concentrations suggested that the air pollution prevention and control in beijing has just won initial success. (c) 2017 elsevier ltd. all rights reserved. |
| WOS关键词 | PARTICULATE MATTER ; PRECIPITATION ; BIPHENYLS ; REGION ; CYCLE ; HAZE |
| WOS研究方向 | Environmental Sciences & Ecology |
| WOS类目 | Environmental Sciences |
| 语种 | 英语 |
| WOS记录号 | WOS:000425075500046 |
| 出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2178047 |
| 专题 | 高能物理研究所 |
| 通讯作者 | Ma, Ling-Ling; Xu, Dian-Dou |
| 作者单位 | 1.Chinese Acad Sci, Beijing Engn Res Ctr Radiog Techn & Equipment, Inst High Energy Physids, Beijing 100049, Peoples R China 2.Univ Chinese Acad Sci, Sch Nucl Sci & Technol, Beijing 100049, Peoples R China 3.Hirosaki Univ, Inst Radiat Emergency Med, Dept Radiat Chem, 66-1 Hon Cho, Hirosaki, Aomori 0368564, Japan 4.Chinese Acad Sci, Inst High Energy Phys, Beijing Synchrotron Radiat Facil, Beijing 100049, Peoples R China 5.Beijing Union Univ, Coll Biochem Engn, Beijing 100023, Peoples R China 6.Beijing North Energy Conservat & Environm Protect, Beijing 100070, Peoples R China |
| 推荐引用方式 GB/T 7714 | Ouyang, Jie,Yang, Guo-Sheng,Ma, Ling-Ling,et al. Chlorine levels and species in fine and size resolved atmospheric particles by x-ray absorption near-edge structure spectroscopy analysis in beijing, china[J]. Chemosphere,2018,196:393-401. |
| APA | Ouyang, Jie.,Yang, Guo-Sheng.,Ma, Ling-Ling.,Luo, Min.,Zheng, Lei.,...&Xu, Dian-Dou.(2018).Chlorine levels and species in fine and size resolved atmospheric particles by x-ray absorption near-edge structure spectroscopy analysis in beijing, china.Chemosphere,196,393-401. |
| MLA | Ouyang, Jie,et al."Chlorine levels and species in fine and size resolved atmospheric particles by x-ray absorption near-edge structure spectroscopy analysis in beijing, china".Chemosphere 196(2018):393-401. |
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来源：高能物理研究所
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