Fabrication of a single-atom platinum catalyst for the hydrogen evolution reaction: a new protocol by utilization of hxmoo3-x with plasmon resonance
文献类型:期刊论文
作者 | Liu, Wei1; Xu, Qun1; Yan, Pengfei1; Chen, Jun2; Du, Yi2; Chu, Shengqi3; Wang, Jiaou3 |
刊名 | Chemcatchem
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出版日期 | 2018-03-07 |
卷号 | 10期号:5页码:946-950 |
关键词 | Amorphous materials Hydrogen Molybdenum Surface plasmon resonance Single-atom catalysts |
ISSN号 | 1867-3880 |
DOI | 10.1002/cctc.201701777 |
通讯作者 | Xu, qun(qunxu@zzu.edu.cn) |
英文摘要 | Single-atom catalysts (sacs) play a key role in many chemical processes owing to highly desirable atom efficiency, but the challenging synthesis of these catalysts limits their commercialization and application on a large scale. herein, we report a facile strategy to integrate atomic pt into richly deficient moo3-x. the core of the experimental strategy was the fabrication and utilization of hxmoo3-x with plasmon resonance that contained intercalated h+. the obtained catalyst was found to possess remarkable electrocatalytic activity toward the hydrogen evolution reaction that was even comparable to that of commercial pt/c, whereas the amount of pt used was reduced to only 10% of the amount of commercial pt/c used. therefore, this work not only supplies a new synthesis route to sacs but also reveals the potential relation between plasmon resonance materials and the fabrication of single-atom catalysts. |
WOS关键词 | CO OXIDATION ; EFFICIENT ; NANOSHEETS ; PERFORMANCE ; ALPHA-MOO3 ; GRAPHENE ; CLUSTERS ; SURFACE ; H-MOO3 ; WATER |
WOS研究方向 | Chemistry |
WOS类目 | Chemistry, Physical |
语种 | 英语 |
WOS记录号 | WOS:000426844600009 |
出版者 | WILEY-V C H VERLAG GMBH |
URI标识 | http://www.irgrid.ac.cn/handle/1471x/2178069 |
专题 | 高能物理研究所 |
通讯作者 | Xu, Qun |
作者单位 | 1.Zhengzhou Univ, Coll Mat Sci & Engn, 75 Daxue North Rd, Zhengzhou 450052, Henan, Peoples R China 2.Univ Wollongong, Intelligent Polymer Res Inst, Australian Inst Innovat Mat, Innovat Campus,Northfields Ave, Wollongong, NSW 2500, Australia 3.Chinese Acad Sci, Beijing Synchrotron Radiat Facil, Inst High Energy Phys, 19B Yuquan Rd, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Liu, Wei,Xu, Qun,Yan, Pengfei,et al. Fabrication of a single-atom platinum catalyst for the hydrogen evolution reaction: a new protocol by utilization of hxmoo3-x with plasmon resonance[J]. Chemcatchem,2018,10(5):946-950. |
APA | Liu, Wei.,Xu, Qun.,Yan, Pengfei.,Chen, Jun.,Du, Yi.,...&Wang, Jiaou.(2018).Fabrication of a single-atom platinum catalyst for the hydrogen evolution reaction: a new protocol by utilization of hxmoo3-x with plasmon resonance.Chemcatchem,10(5),946-950. |
MLA | Liu, Wei,et al."Fabrication of a single-atom platinum catalyst for the hydrogen evolution reaction: a new protocol by utilization of hxmoo3-x with plasmon resonance".Chemcatchem 10.5(2018):946-950. |
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来源:高能物理研究所
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