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Fabrication of a single-atom platinum catalyst for the hydrogen evolution reaction: a new protocol by utilization of hxmoo3-x with plasmon resonance

文献类型:期刊论文

作者Liu, Wei1; Xu, Qun1; Yan, Pengfei1; Chen, Jun2; Du, Yi2; Chu, Shengqi3; Wang, Jiaou3
刊名Chemcatchem
出版日期2018-03-07
卷号10期号:5页码:946-950
关键词Amorphous materials Hydrogen Molybdenum Surface plasmon resonance Single-atom catalysts
ISSN号1867-3880
DOI10.1002/cctc.201701777
通讯作者Xu, qun(qunxu@zzu.edu.cn)
英文摘要Single-atom catalysts (sacs) play a key role in many chemical processes owing to highly desirable atom efficiency, but the challenging synthesis of these catalysts limits their commercialization and application on a large scale. herein, we report a facile strategy to integrate atomic pt into richly deficient moo3-x. the core of the experimental strategy was the fabrication and utilization of hxmoo3-x with plasmon resonance that contained intercalated h+. the obtained catalyst was found to possess remarkable electrocatalytic activity toward the hydrogen evolution reaction that was even comparable to that of commercial pt/c, whereas the amount of pt used was reduced to only 10% of the amount of commercial pt/c used. therefore, this work not only supplies a new synthesis route to sacs but also reveals the potential relation between plasmon resonance materials and the fabrication of single-atom catalysts.
WOS关键词CO OXIDATION ; EFFICIENT ; NANOSHEETS ; PERFORMANCE ; ALPHA-MOO3 ; GRAPHENE ; CLUSTERS ; SURFACE ; H-MOO3 ; WATER
WOS研究方向Chemistry
WOS类目Chemistry, Physical
语种英语
WOS记录号WOS:000426844600009
出版者WILEY-V C H VERLAG GMBH
URI标识http://www.irgrid.ac.cn/handle/1471x/2178069
专题高能物理研究所
通讯作者Xu, Qun
作者单位1.Zhengzhou Univ, Coll Mat Sci & Engn, 75 Daxue North Rd, Zhengzhou 450052, Henan, Peoples R China
2.Univ Wollongong, Intelligent Polymer Res Inst, Australian Inst Innovat Mat, Innovat Campus,Northfields Ave, Wollongong, NSW 2500, Australia
3.Chinese Acad Sci, Beijing Synchrotron Radiat Facil, Inst High Energy Phys, 19B Yuquan Rd, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Liu, Wei,Xu, Qun,Yan, Pengfei,et al. Fabrication of a single-atom platinum catalyst for the hydrogen evolution reaction: a new protocol by utilization of hxmoo3-x with plasmon resonance[J]. Chemcatchem,2018,10(5):946-950.
APA Liu, Wei.,Xu, Qun.,Yan, Pengfei.,Chen, Jun.,Du, Yi.,...&Wang, Jiaou.(2018).Fabrication of a single-atom platinum catalyst for the hydrogen evolution reaction: a new protocol by utilization of hxmoo3-x with plasmon resonance.Chemcatchem,10(5),946-950.
MLA Liu, Wei,et al."Fabrication of a single-atom platinum catalyst for the hydrogen evolution reaction: a new protocol by utilization of hxmoo3-x with plasmon resonance".Chemcatchem 10.5(2018):946-950.

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