Ni2p(o)/fe2p(o) interface can boost oxygen evolution electrocatalysis
文献类型：期刊论文
| 作者 | Liu, Peng Fei1; Li, Xu1; Yang, Shuang1; Zu, Meng Yang1; Liu, Porun2; Zhang, Bo3; Zheng, Li Rong4; Zhao, Huijun2; Yang, Hua Gui1 |
| 刊名 | Acs energy letters
 |
| 出版日期 | 2017-10-01 |
| 卷号 | 2期号:10页码:2257-2263 |
| ISSN号 | 2380-8195 |
| DOI | 10.1021/acsenergylett.7b00638 |
| 通讯作者 | Yang, hua gui(hgyang@ecust.edu.cn) |
| 英文摘要 | Oxygen evolution reaction (oer) plays a paramount role in renewable energy technologies. however, the slow kinetics of oer seriously limits the overall performance and commercialization. here, we rationally design a metallic ni2p/fe2p interface, which can be in situ oxidized to a ni2p(o)/fe2p(o) interface to enhance oer efficiency, with active doped oxyhydroxides and phosphates on the surface and conductive phosphide in the bulk. the resulting catalysts require a low overpotential of 179 mv to achieve a current density of 10 ma/cm(2) (without ir compensation) and can continuously drive oer for 120 h without any obvious degradation, which rivals most reported oer catalysts. these results suggest that we are able to design multicomponent metallic precatalysts to construct most active surface layers and conductive bulks, further boosting oer performance for real-world electrolysis utilization. |
| WOS关键词 | LAYERED DOUBLE HYDROXIDE ; ELECTROCHEMICAL WATER OXIDATION ; EVOLVING CATALYST ; EFFICIENT ; HYDROGEN ; NANOSHEETS ; OXIDE ; NIFE ; IDENTIFICATION ; PHOSPHIDE |
| WOS研究方向 | Chemistry ; Electrochemistry ; Energy & Fuels ; Science & Technology - Other Topics ; Materials Science |
| WOS类目 | Chemistry, Physical ; Electrochemistry ; Energy & Fuels ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
| 语种 | 英语 |
| WOS记录号 | WOS:000415914200009 |
| 出版者 | AMER CHEMICAL SOC |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2178294 |
| 专题 | 高能物理研究所 |
| 通讯作者 | Yang, Hua Gui |
| 作者单位 | 1.East China Univ Sci & Technol, Key Lab Ultrafine Mat, Minist Educ, Sch Mat Sci & Engn, Shanghai 200237, Peoples R China 2.Griffith Univ, Ctr Clean Environm & Energy, Gold Coast Campus, Southport, Qld 4222, Australia 3.Fudan Univ, State Key Lab Mol Engn Polymers, Dept Macromol Sci, Shanghai 200438, Peoples R China 4.Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Liu, Peng Fei,Li, Xu,Yang, Shuang,et al. Ni2p(o)/fe2p(o) interface can boost oxygen evolution electrocatalysis[J]. Acs energy letters,2017,2(10):2257-2263. |
| APA | Liu, Peng Fei.,Li, Xu.,Yang, Shuang.,Zu, Meng Yang.,Liu, Porun.,...&Yang, Hua Gui.(2017).Ni2p(o)/fe2p(o) interface can boost oxygen evolution electrocatalysis.Acs energy letters,2(10),2257-2263. |
| MLA | Liu, Peng Fei,et al."Ni2p(o)/fe2p(o) interface can boost oxygen evolution electrocatalysis".Acs energy letters 2.10(2017):2257-2263. |
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