Degradation of nitrobenzene by trisynergetic attapulgite-supported nanoscale zero-valent iron-biofilm
文献类型：期刊论文
| 作者 | Ma, Xijun1; Zhang, Yingying1; Zhou, Jiuyang1; Xue, Yuanyuan1; Shang, Linjie1; Xie, Xingyong1; Wu, Zhengyan2 ; Zhang, Jing1
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| 刊名 | RESEARCH ON CHEMICAL INTERMEDIATES
 |
| 出版日期 | 2018-11-01 |
| 卷号 | 44期号:11页码:6963-6977 |
| ISSN号 | 0922-6168 |
| 关键词 | Nitrobenzene Attapulgite Nanoscale zero-valent iron Biomembrane Polyvinyl alcohol |
| DOI | 10.1007/s11164-018-3534-6 |
| 通讯作者 | Zhang, Jing(zhangjing860321@hyit.edu.cn) |
| 英文摘要 | A trisynergetic system (AFB) of nanoscale zero-valent iron (NI)-biofilm supported on attapulgite (ATP) was used to degrade nitrobenzene (NTB) in aqueous solution. We first synthesized a nanocomposite of ATP, polyvinyl alcohol, and NI as the growth carrier (AP-NI) for the biofilm. The activity of the biofilm was determined after its successful application, and the microorganisms were domesticated using NTB wastewater. The specific surface area of the AP-NI carrier was 158m(2)/g, much higher than that of the traditional carrier polyvinyl alcohol (30.1m(2)/g). AP-NI could be evenly distributed in water rather than settling, due to its average density of 0.647g/m(3). Additionally, the reductive efficiency of AP-NI towards NTB was about 91%, providing good support for the subsequent construction of the biofilm. Scanning electron microscopy (SEM) results indicated that the microorganisms were dominated by globular bacteria after acclimation, and could completely degrade 8mg/L NTB in 24h with high activity. The microbial activity depended more strongly on the choice of carbon source. Finally, polymerase chain reaction denaturing gradient gel electrophoresis (PCR-DGGE) technology was used to analyze the microbial community structure and 16S ribosomal DNA (rDNA) sequence. The NTB degradation mechanism of the trisynergetic system revealed a mainly aerobic pathway with an iron cycle. |
| WOS关键词 | GROUNDWATER REMEDIATION ; AQUEOUS-SOLUTION ; WASTE-WATER ; NANOPARTICLES ; REDUCTION ; REMOVAL ; BIODEGRADATION ; SCALE ; NZVI ; PH |
| 资助项目 | National Natural Science Foundation of China[41301048] ; Science and Technology Project of Huai'an[2015008] ; Social Development Projects of Huai'an[HAS2014020] ; Open Fund of Jiangsu Provincial Engineering Laboratory for Advanced Materials of Salt Chemical Industry[SF201702-2] ; Practice Innovation Program Project of College Students in Jiangsu Province[201725013XJ] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| 出版者 | SPRINGER |
| WOS记录号 | WOS:000449307900033 |
| 资助机构 | National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Science and Technology Project of Huai'an ; Science and Technology Project of Huai'an ; Science and Technology Project of Huai'an ; Science and Technology Project of Huai'an ; Science and Technology Project of Huai'an ; Science and Technology Project of Huai'an ; 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| 源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/34393]  |
| 专题 | 合肥物质科学研究院_中科院强磁场科学中心 合肥物质科学研究院_技术生物与农业工程研究所 |
| 通讯作者 | Zhang, Jing |
| 作者单位 | 1.Huaiyin Inst Technol, Sch Chem Engn, Jiangsu Prov Engn Lab Adv Mat Salt Chem Ind, Huaian 223003, Peoples R China 2.Chinese Acad Sci, Hefei Inst Phys Sci, Key Lab High Magnet Field & Ion Beam Phys Biol, Hefei 230031, Peoples R China |
| 推荐引用方式 GB/T 7714 | Ma, Xijun,Zhang, Yingying,Zhou, Jiuyang,et al. Degradation of nitrobenzene by trisynergetic attapulgite-supported nanoscale zero-valent iron-biofilm[J]. RESEARCH ON CHEMICAL INTERMEDIATES,2018,44(11):6963-6977. |
| APA | Ma, Xijun.,Zhang, Yingying.,Zhou, Jiuyang.,Xue, Yuanyuan.,Shang, Linjie.,...&Zhang, Jing.(2018).Degradation of nitrobenzene by trisynergetic attapulgite-supported nanoscale zero-valent iron-biofilm.RESEARCH ON CHEMICAL INTERMEDIATES,44(11),6963-6977. |
| MLA | Ma, Xijun,et al."Degradation of nitrobenzene by trisynergetic attapulgite-supported nanoscale zero-valent iron-biofilm".RESEARCH ON CHEMICAL INTERMEDIATES 44.11(2018):6963-6977. |
入库方式： OAI收割
来源：合肥物质科学研究院
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