Significant enhancement in activity of Pd/TiO2 catalyst for formaldehyde oxidation by Na addition
文献类型:期刊论文
作者 | Li, Yaobin; He, Hong; Zhang, Changbin |
刊名 | CATALYSIS TODAY
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出版日期 | 2017-03-01 |
卷号 | 281期号:0页码:412-417 |
关键词 | Sodium Addition Pd/tio2 Formaldehyde Room Temperature Promoter-metal Interaction |
英文摘要 | Developing an effective material for indoor HCHO elimination at ambient temperature is of great significance. In this work, a series of Pd/TiO2 catalysts with different Na loadings were prepared and tested for their activity in HCHO oxidation. The results indicated that Na addition had a remarkable promotion effect on Pd/TiO2 catalysts for HCHO oxidation, and the optimal Na loading was 2 wt.%. Features of the catalysts including the reducibility, Pd dispersion and valence state of Pd and O were elucidated using a variety of characterization techniques. The results showed that 2.0Na-Pd/TiO2 exhibited more exposure of active Pd sites and contained abundant surface OH groups, giving it the best HCHO catalytic oxidation performance of the studied catalysts. The 2.0Na-Pd/TiO2 catalyst also had high resistance to effects of space velocity and relative humidity (RH), maintaining high HCHO conversion over a wide gas hourly space velocity range of 80,000-190,000h(-1) and RH of 25%-65%. (C) 2016 Elsevier B.V. All rights reserved. |
源URL | [http://ir.rcees.ac.cn/handle/311016/39211] ![]() |
专题 | 生态环境研究中心_大气污染控制中心 |
推荐引用方式 GB/T 7714 | Li, Yaobin,He, Hong,Zhang, Changbin. Significant enhancement in activity of Pd/TiO2 catalyst for formaldehyde oxidation by Na addition[J]. CATALYSIS TODAY,2017,281(0):412-417. |
APA | Li, Yaobin,He, Hong,&Zhang, Changbin.(2017).Significant enhancement in activity of Pd/TiO2 catalyst for formaldehyde oxidation by Na addition.CATALYSIS TODAY,281(0),412-417. |
MLA | Li, Yaobin,et al."Significant enhancement in activity of Pd/TiO2 catalyst for formaldehyde oxidation by Na addition".CATALYSIS TODAY 281.0(2017):412-417. |
入库方式: OAI收割
来源:生态环境研究中心
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