Constructing SrTiO3-TiO2 Heterogeneous Hollow Multi-shelled Structures for Enhanced Solar Water Splitting
文献类型：期刊论文
| 作者 | Wei, Yanze1,2; Wang, Jiangyan2; Yu, Ranbo1; Wan, Jiawei2; Wang, Dan2 |
| 刊名 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
 |
| 出版日期 | 2019-01-28 |
| 卷号 | 58期号:5页码:1422-1426 |
| 关键词 | heterostructures hollow structures multiple shells photocatalysis solar water-splitting |
| ISSN号 | 1433-7851 |
| DOI | 10.1002/anie.201812364 |
| 英文摘要 | Constructing hollow multi-shelled structures (HoMSs) has a significant effect on promoting light absorption property of catalysts and enhancing their performance in solar energy conversion applications. A facile hydrothermal method is used to design the SrTiO3-TiO2 heterogeneous HoMSs by hydrothermal crystallization of SrTiO3 on the surface of the TiO2 HoMSs, which will realize a full coverage of SrTiO3 on the TiO2 surface and construct the SrTiO3/TiO2 junctions. The broccoli-like SrTiO3-TiO2 heterogeneous HoMSs exhibited a fourfold higher overall water splitting performance of 10.6 mu mol h(-1) for H-2 production and 5.1 mu mol h(-1) for O-2 evolution than that of SrTiO3 nanoparticles and the apparent quantum efficiency (AQE) of 8.6% at 365 nm, which can be mainly attributed to 1) HoMS increased the light absorption ability of the constructed photocatalysts and 2) the SrTiO3-TiO2 junctions boosted the separation efficiency of the photo-generated charge carriers. |
| WOS关键词 | Z-SCHEME ; MICROSPHERES ; EFFICIENT ; PHOTOCATALYST ; ADSORPTION |
| 资助项目 | National Natural Science Foundation of China[51472025] ; National Natural Science Foundation of China[21671016] ; National Natural Science Foundation of China[51872024] ; National Natural Science Foundation of China[21590795] ; National Natural Science Foundation of China[21820102002] ; National Natural Science Foundation of China[51802306] ; Foundation for CAS Interdisciplinary Innovation Team ; Chinese Academy of Sciences[YZ201623] ; Queensland-Chinese Academy of Sciences Collaborative Science Fund[122111KYSB20170001] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000458826100027 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 资助机构 | National Natural Science Foundation of China ; Foundation for CAS Interdisciplinary Innovation Team ; Chinese Academy of Sciences ; Queensland-Chinese Academy of Sciences Collaborative Science Fund |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/27989]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Yu, Ranbo; Wan, Jiawei; Wang, Dan |
| 作者单位 | 1.Univ Sci & Technol Beijing, Sch Met & Ecol Engn, Dept Phys Chem, 30 Xueyuan Rd, Beijing 100083, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, 1 North 2nd St, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wei, Yanze,Wang, Jiangyan,Yu, Ranbo,et al. Constructing SrTiO3-TiO2 Heterogeneous Hollow Multi-shelled Structures for Enhanced Solar Water Splitting[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2019,58(5):1422-1426. |
| APA | Wei, Yanze,Wang, Jiangyan,Yu, Ranbo,Wan, Jiawei,&Wang, Dan.(2019).Constructing SrTiO3-TiO2 Heterogeneous Hollow Multi-shelled Structures for Enhanced Solar Water Splitting.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,58(5),1422-1426. |
| MLA | Wei, Yanze,et al."Constructing SrTiO3-TiO2 Heterogeneous Hollow Multi-shelled Structures for Enhanced Solar Water Splitting".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 58.5(2019):1422-1426. |
入库方式： OAI收割
来源：过程工程研究所
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